Abstract

We demonstrate a high repetition-rate, single-cycle THz source with a maximum average power of 1.35 mW, operating at a center frequency of 2 THz. This result was obtained by optical rectification (OR) in GaP using an amplifier-free, nonlinearly compressed modelocked thin-disk oscillator based on Yb:YAG, delivering 8.4 µJ pulses with 88 fs duration at a repetition rate of 13.4 MHz, resulting in driving pulses for OR with 112 W average power and 80 MW peak power. To the best of our knowledge, our result represents the highest average power so far achieved with OR in GaP. The demonstrated performance is very attractive for improving current linear THz time-domain spectroscopy experiments, which are currently restricted by low signal-to-noise ratio and long measurement times.

© 2019 Optical Society of America under the terms of the OSA Open Access Publishing Agreement

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2019 (3)

C.-L. Tsai, F. Meyer, A. Omar, Y. Wang, A.-Y. Liang, C.-H. Lu, M. Hoffmann, S.-D. Yang, and C. J. Saraceno, “Efficient nonlinear compression of a mode-locked thin-disk oscillator to 27fs at 98W average power,” Opt. Lett. 44(17), 4115–4118 (2019).
[Crossref]

C. Hoberg, P. Balzerowski, and M. Havenith, “Integration of a rapid scanning technique into THz time-domain spectrometers for nonlinear THz spectroscopy measurements,” AIP Adv. 9(3), 035348 (2019).
[Crossref]

R. B. Kohlhaas, S. Breuer, S. Nellen, L. Liebermeister, M. Schell, M. P. Semtsiv, W. T. Masselink, and B. Globisch, “Photoconductive terahertz detectors with 105 dB peak dynamic range made of rhodium doped InGaAs,” Appl. Phys. Lett. 114(22), 221103 (2019).
[Crossref]

2018 (5)

2017 (5)

2016 (3)

J. Schulte, T. Sartorius, J. Weitenberg, A. Vernaleken, and P. Russbueldt, “Nonlinear pulse compression in a multi-pass cell,” Opt. Lett. 41(19), 4511 (2016).
[Crossref]

B. Green, S. Kovalev, V. Asgekar, G. Geloni, U. Lehnert, T. Golz, M. Kuntzsch, C. Bauer, J. Hauser, J. Voigtlaender, B. Wustmann, I. Koesterke, M. Schwarz, M. Freitag, A. Arnold, J. Teichert, M. Justus, W. Seidel, C. Ilgner, N. Awari, D. Nicoletti, S. Kaiser, Y. Laplace, S. Rajasekaran, L. Zhang, S. Winnerl, H. Schneider, G. Schay, I. Lorincz, A. A. Rauscher, I. Radu, S. Mährlein, T. H. Kim, J. S. Lee, T. Kampfrath, S. Wall, J. Heberle, A. Malnasi-Csizmadia, A. Steiger, A. S. Müller, M. Helm, U. Schramm, T. Cowan, P. Michel, A. Cavalleri, A. S. Fisher, N. Stojanovic, and M. Gensch, “High-Field High-Repetition-Rate Sources for the Coherent THz Control of Matter,” Sci. Rep. 6(1), 22256 (2016).
[Crossref]

M. Müller, M. Kienel, A. Klenke, T. Gottschall, E. Shestaev, M. Plötner, J. Limpert, and A. Tünnermann, “1 kW 1 mJ eight-channel ultrafast fiber laser,” Opt. Lett. 41(15), 3439 (2016).
[Crossref]

2014 (3)

2013 (3)

J. Li, L. Chai, J. Shi, F. Liu, B. Liu, B. Xu, M. Hu, Y. Li, Q. Xing, C. Wang, A. B. Fedotov, and A. M. Zheltikov, “Generation of 0.3 mW high-power broadband terahertz pulses from GaP crystal pumped by negatively chirped femtosecond laser pulses,” Laser Phys. Lett. 10(12), 125404 (2013).
[Crossref]

S.-W. Huang, E. Granados, W. R. Huang, K.-H. Hong, L. E. Zapata, and F. X. Kärtner, “High conversion efficiency, high energy terahertz pulses by optical rectification in cryogenically cooled lithium niobate,” Opt. Lett. 38(5), 796 (2013).
[Crossref]

J. Savolainen, S. Ahmed, and P. Hamm, “Two-dimensional Raman-terahertz spectroscopy of water,” Proc. Natl. Acad. Sci. 110(51), 20402–20407 (2013).
[Crossref]

2012 (2)

2011 (3)

J.-P. Negel, R. Hegenbarth, A. Steinmann, B. Metzger, F. Hoos, and H. Giessen, “Compact and cost-effective scheme for THz generation via optical rectification in GaP and GaAs using novel fs laser oscillators,” Appl. Phys. B: Lasers Opt. 103(1), 45–50 (2011).
[Crossref]

C. P. Hauri, C. Ruchert, C. Vicario, and F. Ardana, “Strong-field single-cycle THz pulses generated in an organic crystal,” Appl. Phys. Lett. 99(16), 161116 (2011).
[Crossref]

H. Hirori, A. Doi, F. Blanchard, and K. Tanaka, “Single-cycle terahertz pulses with amplitudes exceeding 1 MV/cm generated by optical rectification in LiNbO3,” Appl. Phys. Lett. 98(9), 091106 (2011).
[Crossref]

2010 (2)

2009 (1)

J. Liu and X. C. Zhang, “Birefringence and absorption coefficients of alpha barium borate in terahertz range,” J. Appl. Phys. 106(2), 023107 (2009).
[Crossref]

2008 (2)

K. Y. Kim, A. J. Taylor, J. H. Glownia, and G. Rodriguez, “Coherent control of terahertz supercontinuum generation in ultrafast laser–gas interactions,” Nat. Photonics 2(10), 605–609 (2008).
[Crossref]

S. J. Kim, B. Born, M. Havenith, and M. Gruebele, “Real-Time Detection of Protein-Water Dynamics upon Protein Folding by Terahertz Absorption Spectroscopy,” Angew. Chem., Int. Ed. 47(34), 6486–6489 (2008).
[Crossref]

2007 (1)

2004 (1)

Y. J. Ding, “Quasi-Single-Cycle Terahertz Pulses Based on Broadband-Phase-Matched Difference-Frequency Generation in Second-Order Nonlinear Medium: High Output Powers and Conversion Efficiencies,” IEEE J. Sel. Top. Quantum Electron. 10(5), 1171–1179 (2004).
[Crossref]

2002 (1)

1997 (1)

R. Trebino, K. W. DeLong, D. N. Fittinghoff, J. N. Sweetser, M. A. Krumbügel, B. A. Richman, and D. J. Kane, “Measuring ultrashort laser pulses in the time-frequency domain using frequency-resolved optical gating,” Rev. Sci. Instrum. 68(9), 3277–3295 (1997).
[Crossref]

1964 (1)

Ahmed, S.

J. Savolainen, S. Ahmed, and P. Hamm, “Two-dimensional Raman-terahertz spectroscopy of water,” Proc. Natl. Acad. Sci. 110(51), 20402–20407 (2013).
[Crossref]

Almasi, G.

Aoki, K.

K. Aoki, J. Savolainen, and M. Havenith, “Broadband terahertz pulse generation by optical rectification in GaP crystals,” Appl. Phys. Lett. 110(20), 201103 (2017).
[Crossref]

Ardana, F.

C. P. Hauri, C. Ruchert, C. Vicario, and F. Ardana, “Strong-field single-cycle THz pulses generated in an organic crystal,” Appl. Phys. Lett. 99(16), 161116 (2011).
[Crossref]

Arnold, A.

B. Green, S. Kovalev, V. Asgekar, G. Geloni, U. Lehnert, T. Golz, M. Kuntzsch, C. Bauer, J. Hauser, J. Voigtlaender, B. Wustmann, I. Koesterke, M. Schwarz, M. Freitag, A. Arnold, J. Teichert, M. Justus, W. Seidel, C. Ilgner, N. Awari, D. Nicoletti, S. Kaiser, Y. Laplace, S. Rajasekaran, L. Zhang, S. Winnerl, H. Schneider, G. Schay, I. Lorincz, A. A. Rauscher, I. Radu, S. Mährlein, T. H. Kim, J. S. Lee, T. Kampfrath, S. Wall, J. Heberle, A. Malnasi-Csizmadia, A. Steiger, A. S. Müller, M. Helm, U. Schramm, T. Cowan, P. Michel, A. Cavalleri, A. S. Fisher, N. Stojanovic, and M. Gensch, “High-Field High-Repetition-Rate Sources for the Coherent THz Control of Matter,” Sci. Rep. 6(1), 22256 (2016).
[Crossref]

Asgekar, V.

B. Green, S. Kovalev, V. Asgekar, G. Geloni, U. Lehnert, T. Golz, M. Kuntzsch, C. Bauer, J. Hauser, J. Voigtlaender, B. Wustmann, I. Koesterke, M. Schwarz, M. Freitag, A. Arnold, J. Teichert, M. Justus, W. Seidel, C. Ilgner, N. Awari, D. Nicoletti, S. Kaiser, Y. Laplace, S. Rajasekaran, L. Zhang, S. Winnerl, H. Schneider, G. Schay, I. Lorincz, A. A. Rauscher, I. Radu, S. Mährlein, T. H. Kim, J. S. Lee, T. Kampfrath, S. Wall, J. Heberle, A. Malnasi-Csizmadia, A. Steiger, A. S. Müller, M. Helm, U. Schramm, T. Cowan, P. Michel, A. Cavalleri, A. S. Fisher, N. Stojanovic, and M. Gensch, “High-Field High-Repetition-Rate Sources for the Coherent THz Control of Matter,” Sci. Rep. 6(1), 22256 (2016).
[Crossref]

Aslani, F.

Awari, N.

B. Green, S. Kovalev, V. Asgekar, G. Geloni, U. Lehnert, T. Golz, M. Kuntzsch, C. Bauer, J. Hauser, J. Voigtlaender, B. Wustmann, I. Koesterke, M. Schwarz, M. Freitag, A. Arnold, J. Teichert, M. Justus, W. Seidel, C. Ilgner, N. Awari, D. Nicoletti, S. Kaiser, Y. Laplace, S. Rajasekaran, L. Zhang, S. Winnerl, H. Schneider, G. Schay, I. Lorincz, A. A. Rauscher, I. Radu, S. Mährlein, T. H. Kim, J. S. Lee, T. Kampfrath, S. Wall, J. Heberle, A. Malnasi-Csizmadia, A. Steiger, A. S. Müller, M. Helm, U. Schramm, T. Cowan, P. Michel, A. Cavalleri, A. S. Fisher, N. Stojanovic, and M. Gensch, “High-Field High-Repetition-Rate Sources for the Coherent THz Control of Matter,” Sci. Rep. 6(1), 22256 (2016).
[Crossref]

Baer, C. R. E.

Balzerowski, P.

C. Hoberg, P. Balzerowski, and M. Havenith, “Integration of a rapid scanning technique into THz time-domain spectrometers for nonlinear THz spectroscopy measurements,” AIP Adv. 9(3), 035348 (2019).
[Crossref]

Bauer, C.

B. Green, S. Kovalev, V. Asgekar, G. Geloni, U. Lehnert, T. Golz, M. Kuntzsch, C. Bauer, J. Hauser, J. Voigtlaender, B. Wustmann, I. Koesterke, M. Schwarz, M. Freitag, A. Arnold, J. Teichert, M. Justus, W. Seidel, C. Ilgner, N. Awari, D. Nicoletti, S. Kaiser, Y. Laplace, S. Rajasekaran, L. Zhang, S. Winnerl, H. Schneider, G. Schay, I. Lorincz, A. A. Rauscher, I. Radu, S. Mährlein, T. H. Kim, J. S. Lee, T. Kampfrath, S. Wall, J. Heberle, A. Malnasi-Csizmadia, A. Steiger, A. S. Müller, M. Helm, U. Schramm, T. Cowan, P. Michel, A. Cavalleri, A. S. Fisher, N. Stojanovic, and M. Gensch, “High-Field High-Repetition-Rate Sources for the Coherent THz Control of Matter,” Sci. Rep. 6(1), 22256 (2016).
[Crossref]

Baum, P.

Beck, M.

Blanchard, F.

H. Hirori, A. Doi, F. Blanchard, and K. Tanaka, “Single-cycle terahertz pulses with amplitudes exceeding 1 MV/cm generated by optical rectification in LiNbO3,” Appl. Phys. Lett. 98(9), 091106 (2011).
[Crossref]

Bonn, M.

Born, B.

S. J. Kim, B. Born, M. Havenith, and M. Gruebele, “Real-Time Detection of Protein-Water Dynamics upon Protein Folding by Terahertz Absorption Spectroscopy,” Angew. Chem., Int. Ed. 47(34), 6486–6489 (2008).
[Crossref]

Breuer, S.

R. B. Kohlhaas, S. Breuer, S. Nellen, L. Liebermeister, M. Schell, M. P. Semtsiv, W. T. Masselink, and B. Globisch, “Photoconductive terahertz detectors with 105 dB peak dynamic range made of rhodium doped InGaAs,” Appl. Phys. Lett. 114(22), 221103 (2019).
[Crossref]

Bromberger, H.

Brons, J.

Butler, T.

J. Xu, B. Globisch, C. Hofer, N. Lilienfein, T. Butler, N. Karpowicz, and I. Pupeza, “Three-octave terahertz pulses from optical rectification of 20 fs, 1 μ m, 78 MHz pulses in GaP,” J. Phys. B: At., Mol. Opt. Phys. 51(15), 154002 (2018).
[Crossref]

Cakmakyapan, S.

N. T. Yardimci, S. Cakmakyapan, S. Hemmati, and M. Jarrahi, “A High-Power Broadband Terahertz Source Enabled by Three-Dimensional Light Confinement in a Plasmonic Nanocavity,” Sci. Rep. 7(1), 4166 (2017).
[Crossref]

Cartella, A.

Cavalleri, A.

B. Liu, H. Bromberger, A. Cartella, T. Gebert, M. Först, and A. Cavalleri, “Generation of narrowband, high-intensity, carrier-envelope phase-stable pulses tunable between 4 and 18 THz,” Opt. Lett. 42(1), 129 (2017).
[Crossref]

B. Green, S. Kovalev, V. Asgekar, G. Geloni, U. Lehnert, T. Golz, M. Kuntzsch, C. Bauer, J. Hauser, J. Voigtlaender, B. Wustmann, I. Koesterke, M. Schwarz, M. Freitag, A. Arnold, J. Teichert, M. Justus, W. Seidel, C. Ilgner, N. Awari, D. Nicoletti, S. Kaiser, Y. Laplace, S. Rajasekaran, L. Zhang, S. Winnerl, H. Schneider, G. Schay, I. Lorincz, A. A. Rauscher, I. Radu, S. Mährlein, T. H. Kim, J. S. Lee, T. Kampfrath, S. Wall, J. Heberle, A. Malnasi-Csizmadia, A. Steiger, A. S. Müller, M. Helm, U. Schramm, T. Cowan, P. Michel, A. Cavalleri, A. S. Fisher, N. Stojanovic, and M. Gensch, “High-Field High-Repetition-Rate Sources for the Coherent THz Control of Matter,” Sci. Rep. 6(1), 22256 (2016).
[Crossref]

Celik, M. A.

Chai, L.

J. Li, L. Chai, J. Shi, F. Liu, B. Liu, B. Xu, M. Hu, Y. Li, Q. Xing, C. Wang, A. B. Fedotov, and A. M. Zheltikov, “Generation of 0.3 mW high-power broadband terahertz pulses from GaP crystal pumped by negatively chirped femtosecond laser pulses,” Laser Phys. Lett. 10(12), 125404 (2013).
[Crossref]

Cowan, T.

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J. Xu, B. Globisch, C. Hofer, N. Lilienfein, T. Butler, N. Karpowicz, and I. Pupeza, “Three-octave terahertz pulses from optical rectification of 20 fs, 1 μ m, 78 MHz pulses in GaP,” J. Phys. B: At., Mol. Opt. Phys. 51(15), 154002 (2018).
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B. Green, S. Kovalev, V. Asgekar, G. Geloni, U. Lehnert, T. Golz, M. Kuntzsch, C. Bauer, J. Hauser, J. Voigtlaender, B. Wustmann, I. Koesterke, M. Schwarz, M. Freitag, A. Arnold, J. Teichert, M. Justus, W. Seidel, C. Ilgner, N. Awari, D. Nicoletti, S. Kaiser, Y. Laplace, S. Rajasekaran, L. Zhang, S. Winnerl, H. Schneider, G. Schay, I. Lorincz, A. A. Rauscher, I. Radu, S. Mährlein, T. H. Kim, J. S. Lee, T. Kampfrath, S. Wall, J. Heberle, A. Malnasi-Csizmadia, A. Steiger, A. S. Müller, M. Helm, U. Schramm, T. Cowan, P. Michel, A. Cavalleri, A. S. Fisher, N. Stojanovic, and M. Gensch, “High-Field High-Repetition-Rate Sources for the Coherent THz Control of Matter,” Sci. Rep. 6(1), 22256 (2016).
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B. Green, S. Kovalev, V. Asgekar, G. Geloni, U. Lehnert, T. Golz, M. Kuntzsch, C. Bauer, J. Hauser, J. Voigtlaender, B. Wustmann, I. Koesterke, M. Schwarz, M. Freitag, A. Arnold, J. Teichert, M. Justus, W. Seidel, C. Ilgner, N. Awari, D. Nicoletti, S. Kaiser, Y. Laplace, S. Rajasekaran, L. Zhang, S. Winnerl, H. Schneider, G. Schay, I. Lorincz, A. A. Rauscher, I. Radu, S. Mährlein, T. H. Kim, J. S. Lee, T. Kampfrath, S. Wall, J. Heberle, A. Malnasi-Csizmadia, A. Steiger, A. S. Müller, M. Helm, U. Schramm, T. Cowan, P. Michel, A. Cavalleri, A. S. Fisher, N. Stojanovic, and M. Gensch, “High-Field High-Repetition-Rate Sources for the Coherent THz Control of Matter,” Sci. Rep. 6(1), 22256 (2016).
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R. B. Kohlhaas, S. Breuer, S. Nellen, L. Liebermeister, M. Schell, M. P. Semtsiv, W. T. Masselink, and B. Globisch, “Photoconductive terahertz detectors with 105 dB peak dynamic range made of rhodium doped InGaAs,” Appl. Phys. Lett. 114(22), 221103 (2019).
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Shi, J.

J. Li, L. Chai, J. Shi, F. Liu, B. Liu, B. Xu, M. Hu, Y. Li, Q. Xing, C. Wang, A. B. Fedotov, and A. M. Zheltikov, “Generation of 0.3 mW high-power broadband terahertz pulses from GaP crystal pumped by negatively chirped femtosecond laser pulses,” Laser Phys. Lett. 10(12), 125404 (2013).
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B. Green, S. Kovalev, V. Asgekar, G. Geloni, U. Lehnert, T. Golz, M. Kuntzsch, C. Bauer, J. Hauser, J. Voigtlaender, B. Wustmann, I. Koesterke, M. Schwarz, M. Freitag, A. Arnold, J. Teichert, M. Justus, W. Seidel, C. Ilgner, N. Awari, D. Nicoletti, S. Kaiser, Y. Laplace, S. Rajasekaran, L. Zhang, S. Winnerl, H. Schneider, G. Schay, I. Lorincz, A. A. Rauscher, I. Radu, S. Mährlein, T. H. Kim, J. S. Lee, T. Kampfrath, S. Wall, J. Heberle, A. Malnasi-Csizmadia, A. Steiger, A. S. Müller, M. Helm, U. Schramm, T. Cowan, P. Michel, A. Cavalleri, A. S. Fisher, N. Stojanovic, and M. Gensch, “High-Field High-Repetition-Rate Sources for the Coherent THz Control of Matter,” Sci. Rep. 6(1), 22256 (2016).
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Wustmann, B.

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N. T. Yardimci, S. Cakmakyapan, S. Hemmati, and M. Jarrahi, “A High-Power Broadband Terahertz Source Enabled by Three-Dimensional Light Confinement in a Plasmonic Nanocavity,” Sci. Rep. 7(1), 4166 (2017).
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B. Green, S. Kovalev, V. Asgekar, G. Geloni, U. Lehnert, T. Golz, M. Kuntzsch, C. Bauer, J. Hauser, J. Voigtlaender, B. Wustmann, I. Koesterke, M. Schwarz, M. Freitag, A. Arnold, J. Teichert, M. Justus, W. Seidel, C. Ilgner, N. Awari, D. Nicoletti, S. Kaiser, Y. Laplace, S. Rajasekaran, L. Zhang, S. Winnerl, H. Schneider, G. Schay, I. Lorincz, A. A. Rauscher, I. Radu, S. Mährlein, T. H. Kim, J. S. Lee, T. Kampfrath, S. Wall, J. Heberle, A. Malnasi-Csizmadia, A. Steiger, A. S. Müller, M. Helm, U. Schramm, T. Cowan, P. Michel, A. Cavalleri, A. S. Fisher, N. Stojanovic, and M. Gensch, “High-Field High-Repetition-Rate Sources for the Coherent THz Control of Matter,” Sci. Rep. 6(1), 22256 (2016).
[Crossref]

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Figures (4)

Fig. 1.
Fig. 1. Complete experimental setup consisting of the modelocked thin-disk laser (a), Herriott type MPC and dispersive mirrors (b), as well as THz generation and detection setup (c).
Fig. 2.
Fig. 2. Compression results measured with SHG-FROG. a) and b) Measured and retrieved traces. c) Retrieved, simulated and measured spectrum and spectral phase. The unbroadened oscillator spectrum is shown for reference in grey. d) Retrieved pulse intensity and phase in the time domain. The transform limit obtained from the measured spectrum is shown for comparison. The inset shows the beam profile used for THz generation at the position of the GaP crystal.
Fig. 3.
Fig. 3. EOS results for different crystal thicknesses under purged conditions. a) Measured electric fields. The amplitudes are to scale with respect to each other, however offset from each other for better visibility. The inset shows the measured THz focus for the 2 mm crystal. b) Corresponding spectra. A spectrum obtained with a 580-fs driving pulse directly from the oscillator in a 2 mm crystal is shown for comparison. c) Same spectra as in b) on a logarithmic scale. A dynamic range better than 60 dB is achieved by averaging 50 traces.
Fig. 4.
Fig. 4. THz power as a function of pump power. a) Optimization for different 1/e2 pump-beam diameters used with the 1 mm crystal. b) Variation of the crystal thickness for a 950 µm spot size.

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