Abstract

Improving the optoelectronic characteristics of organic-inorganic perovskites is crucial for fabrication of functional devices. Herein, we demonstrate that the optoelectronic properties of 2D organic-inorganic perovskites can be greatly improved by UV-light illumination during growth. The photoluminescence emission of the 2D perovskite exhibits a 3.1-folds increase in intensity, with a decreased trap-assisted recombination. The improved optoelectronic characteristics can be attributed to the high-quality crystallization and lattice expansion induced by the UV-light illumination. Moreover, the optimized 2D perovskites enable the fabrication of photoconductive devices with improved optoelectronic responses. This work indicates that light illumination is a novel and convenient approach for engineering the fabrication of 2D organic-inorganic hybrid perovskites, which advocates great promise for achieving high-performance functional devices.

© 2019 Optical Society of America under the terms of the OSA Open Access Publishing Agreement

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2019 (7)

G. Hu, X. Hong, K. Wang, J. Wu, H.-X. Xu, W. Zhao, W. Liu, S. Zhang, F. Garcia-Vidal, B. Wang, P. Lu, and C.-W. Qiu, “Coherent steering of nonlinear chiral valley photons with a synthetic Au-WS2 metasurface,” Nat. Photonics 13(7), 467–472 (2019).
[Crossref]

X. Li, W. Liu, Y. Song, C. Zhang, H. Long, K. Wang, B. Wang, and P. Lu, “Enhancement of the Second Harmonic Generation from WS2 Monolayers by Cooperating with Dielectric Microspheres,” Adv. Opt. Mater. 7(3), 1801270 (2019).
[Crossref]

M. T. Yu, C. Yi, N. N. Wang, L. D. Zhang, R. M. Zou, Y. F. Tong, H. Chen, Y. Cao, Y. R. He, Y. Wang, M. M. Xu, Y. Liu, Y. Z. Jin, W. Huang, and J. P. Wang, “Control of Barrier Width in Perovskite Multiple Quantum Wells for High Performance Green Light-Emitting Diodes,” Adv. Opt. Mater. 7(3), 1801575 (2019).
[Crossref]

W. J. Wei, X. X. Jiang, L. Y. Dong, W. W. Liu, X. B. Han, Y. Qin, K. Li, W. Li, Z. S. Lin, X. H. Bu, and P. X. Lu, “Regulating Second-Harmonic Generation by van der Waals Interactions in Two-dimensional Lead Halide Perovskite Nanosheets,” J. Am. Chem. Soc. 141(23), 9134–9139 (2019).
[Crossref]

G. Delport, G. Chehade, F. Lédée, H. Diab, C. Milesi-Brault, G. Trippé-Allard, J. Even, J.-S. Lauret, E. Deleporte, and D. Garrot, “Exciton-Exciton Annihilation in Two-Dimensional Halide Perovskites at Room Temperature,” J. Phys. Chem. Lett. 10(17), 5153–5159 (2019).
[Crossref]

D. M. Kinyua, H. Long, X. Y. Xing, S. Njoroge, K. Wang, B. Wang, and P. X. Lu, “Gigahertz acoustic vibrations of Ga-doped ZnO nanoparticle array,” Nanotechnology 30(30), 305201 (2019).
[Crossref]

D. M. Kinyua, L. Niu, H. Long, K. Wang, and B. Wang, “Tuning the photoinduced charge transfer from CdTe quantum dots to ZnO nanofilms through Ga doping,” Opt. Mater. 96, 109311 (2019).
[Crossref]

2018 (17)

H. H. Fang, J. Yang, S. X. Tao, S. Adjokatse, M. E. Kamminga, J. T. Ye, G. R. Blake, J. Even, and M. A. Loi, “Unravelling Light-Induced Degradation of Layered Perovskite Crystals and Design of Efficient Encapsulation for Improved Photostability,” Adv. Funct. Mater. 28(21), 1800305 (2018).
[Crossref]

W. Liu, X. Li, Y. Song, C. Zhang, X. Han, H. Long, B. Wang, K. Wang, and P. Lu, “Cooperative Enhancement of Two-Photon-Absorption-Induced Photoluminescence from a 2D Perovskite-Microsphere Hybrid Dielectric Structure,” Adv. Funct. Mater. 28(26), 1707550 (2018).
[Crossref]

Y. Song, C. Zhang, W. Liu, X. Li, H. Long, K. Wang, B. Wang, and P. Lu, “High-efficiency energy transfer in perovskite heterostructures,” Opt. Express 26(14), 18448–18456 (2018).
[Crossref]

Z. X. Zhang, Z. Long-Hui, X. W. Tong, Y. Gao, C. Xie, Y. H. Tsang, L. B. Luo, and Y. C. Wu, “Ultrafast, Self-Driven, and Air-Stable Photodetectors Based on Multilayer PtSe2/Perovskite Heterojunctions,” J. Phys. Chem. Lett. 9(6), 1185–1194 (2018).
[Crossref]

H. Tsai, R. Asadpour, J. C. Blancon, C. C. Stoumpos, O. Durand, J. W. Strzalka, B. Chen, R. Verduzco, P. M. Ajayan, S. Tretiak, J. Even, M. A. Alam, M. G. Kanatzidis, W. Nie, and A. D. Mohite, “Light-induced lattice expansion leads to high-efficiency perovskite solar cells,” Science 360(6384), 67–70 (2018).
[Crossref]

R. Brenes, C. Eames, V. Bulovic, M. S. Islam, and S. D. Stranks, “The Impact of Atmosphere on the Local Luminescence Properties of Metal Halide Perovskite Grains,” Adv. Mater. 30(15), 1706208 (2018).
[Crossref]

B. Zhao, S. Bai, V. Kim, R. Lamboll, R. Shivanna, F. Auras, J. M. Richter, L. Yang, L. Dai, M. Alsari, X.-J. She, L. Liang, J. Zhang, S. Lilliu, P. Gao, H. J. Snaith, J. Wang, N. C. Greenham, R. H. Friend, and D. Di, “High-efficiency perovskite-polymer bulk heterostructure light-emitting diodes,” Nat. Photonics 12(12), 783–789 (2018).
[Crossref]

H. Xiong, G. DeLuca, Y. Rui, B. Zhang, Y. Li, Q. Zhang, H. Wang, and E. Reichmanis, “Modifying Perovskite Films with Polyvinylpyrrolidone for Ambient-Air-Stable Highly Bendable Solar Cells,” ACS Appl. Mater. Interfaces 10(41), 35385–35394 (2018).
[Crossref]

H. Zhang, Q. Liao, Y. Wu, Z. Zhang, Q. Gao, P. Liu, M. Li, J. Yao, and H. Fu, “2D Ruddlesden-Popper Perovskites Microring Laser Array,” Adv. Mater. 30(15), 1706186 (2018).
[Crossref]

S. Yuan, Z. K. Wang, M. P. Zhuo, Q. S. Tian, Y. Jin, and L. S. Liao, “Self-Assembled High Quality CsPbBr3 Quantum Dot Films toward Highly Efficient Light-Emitting Diodes,” ACS Nano 12(9), 9541–9548 (2018).
[Crossref]

Z. Zhang, D. Schwanz, B. Narayanan, M. Kotiuga, J. A. Dura, M. Cherukara, H. Zhou, J. W. Freeland, J. Li, R. Sutarto, F. He, C. Wu, J. Zhu, Y. Sun, K. Ramadoss, S. S. Nonnenmann, N. Yu, R. Comin, K. M. Rabe, S. Sankaranarayanan, and S. Ramanathan, “Perovskite nickelates as electric-field sensors in salt water,” Nature 553(7686), 68–72 (2018).
[Crossref]

R. Guo, F. Huang, K. Zheng, T. Pullerits, and J. Tian, “CuInSe2 Quantum Dots Hybrid Hole Transfer Layer for Halide Perovskite Photodetectors,” ACS Appl. Mater. Interfaces 10(41), 35656–35663 (2018).
[Crossref]

J. W. Chen, K. Wang, H. Long, X. B. Han, H. B. Hu, W. W. Liu, B. Wang, and P. X. Lu, “Tungsten Disulfide-Gold Nanohole Hybrid Metasurfaces for Nonlinear Metalenses in the Visible Region,” Nano Lett. 18(2), 1344–1350 (2018).
[Crossref]

M. Abdi-Jalebi, Z. Andaji-Garmaroudi, S. Cacovich, C. Stavrakas, B. Philippe, J. M. Richter, M. Alsari, E. P. Booker, E. M. Hutter, A. J. Pearson, S. Lilliu, T. J. Savenije, H. Rensmo, G. Divitini, C. Ducati, R. H. Friend, and S. D. Stranks, “Maximizing and stabilizing luminescence from halide perovskites with potassium passivation,” Nature 555(7697), 497–501 (2018).
[Crossref]

D. Gui, L. Ji, A. Muhammad, W. Li, W. Cai, Y. Li, X. Li, X. Wu, and P. Lu, “Jahn-Teller Effect on Framework Flexibility of Hybrid Organic-Inorganic Perovskites,” J. Phys. Chem. Lett. 9(4), 751–755 (2018).
[Crossref]

S. Manzoor, J. Häusele, K. A. Bush, A. F. Palmstrom, J. Carpenter, Z. J. Yu, S. F. Bent, M. D. McGehee, and Z. C. Holman, “Optical modeling of wide-bandgap perovskite and perovskite/silicon tandem solar cells using complex refractive indices for arbitrary-bandgap perovskite absorbers,” Opt. Express 26(21), 27441–27460 (2018).
[Crossref]

K. T. Cho, Y. Zhang, S. Orlandi, M. Cavazzini, I. Zimmermann, A. Lesch, N. Tabet, G. Pozzi, G. Grancini, and M. K. Nazeeruddin, “Water-Repellent Low-Dimensional Fluorous Perovskite as Interfacial Coating for 20% Efficient Solar Cells,” Nano Lett. 18(9), 5467–5474 (2018).
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2017 (9)

J.-C. Blancon, H. Tsai, W. Nie, C. C. Stoumpos, L. Pedesseau, C. Katan, M. Kepenekian, C. M. M. Soe, K. Appavoo, M. Y. Sfeir, S. Tretiak, P. M. Ajayan, M. G. Kanatzidis, J. Even, J. J. Crochet, and A. D. Mohite, “Extremely efficient internal exciton dissociation through edge states in layered 2D perovskites,” Science 355(6331), 1288–1292 (2017).
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W. Tian, J. Leng, C. Zhao, and S. Jin, “Long-Distance Charge Carrier Funneling in Perovskite Nanowires Enabled by Built-in Halide Gradient,” J. Am. Chem. Soc. 139(2), 579–582 (2017).
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S. Manzeli, D. Ovchinnikov, D. Pasquier, O. V. Yazyev, and A. Kis, “2D transition metal dichalcogenides,” Nat. Rev. Mater. 2(8), 17033 (2017).
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D. W. Ma, Y. P. Fu, L. N. Dang, J. Y. Zhai, I. A. Guzei, and S. Jin, “Single-crystal microplates of two-dimensional organic-inorganic lead halide layered perovskites for optoelectronics,” Nano Res. 10(6), 2117–2129 (2017).
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W. Liu, J. Xing, J. Zhao, X. Wen, K. Wang, P. Lu, and Q. Xiong, “Giant Two-Photon Absorption and Its Saturation in 2D Organic-Inorganic Perovskite,” Adv. Opt. Mater. 5(7), 1601045 (2017).
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A. Ummadisingu, L. Steier, J. Y. Seo, T. Matsui, A. Abate, W. Tress, and M. Gratzel, “The effect of illumination on the formation of metal halide perovskite films,” Nature 545(7653), 208–212 (2017).
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F. Ledee, G. Trippe-Allard, H. Diab, P. Audebert, D. Garrot, J. S. Lauret, and E. Deleporte, “Fast growth of monocrystalline thin films of 2D layered hybrid perovskite,” CrystEngComm 19(19), 2598–2602 (2017).
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C. Bao, Z. Chen, Y. Fang, H. Wei, Y. Deng, X. Xiao, L. Li, and J. Huang, “Low-Noise and Large-Linear-Dynamic-Range Photodetectors Based on Hybrid-Perovskite Thin-Single-Crystals,” Adv. Mater. 29(39), 1703209 (2017).
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H. Sun, T. Lei, W. Tian, F. Cao, J. Xiong, and L. Li, “Self-Powered, Flexible, and Solution-Processable Perovskite Photodetector Based on Low-Cost Carbon Cloth,” Small 13(28), 1701042 (2017).
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2016 (9)

F. Staub, H. Hempel, J. C. Hebig, J. Mock, U. W. Paetzold, U. Rau, T. Unold, and T. Kirchartz, “Beyond Bulk Lifetimes: Insights into Lead Halide Perovskite Films from Time-Resolved Photoluminescence,” Phys. Rev. Appl. 6(4), 044017 (2016).
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J. Ding, H. Fang, Z. Lian, J. Li, Q. Lv, L. Wang, J.-L. Sun, and Q. Yan, “A self-powered photodetector based on a CH3NH3PbI3 single crystal with asymmetric electrodes,” CrystEngComm 18(23), 4405–4411 (2016).
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X. J. Zheng, C. C. Wu, S. K. Jha, Z. Li, K. Zhu, and S. Priya, “Improved Phase Stability of Formamidinium Lead Triiodide Perovskite by Strain Relaxation,” ACS Energy Lett. 1(5), 1014–1020 (2016).
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M. Yuan, L. N. Quan, R. Comin, G. Walters, R. Sabatini, O. Voznyy, S. Hoogland, Y. Zhao, E. M. Beauregard, P. Kanjanaboos, Z. Lu, D. H. Kim, and E. H. Sargent, “Perovskite energy funnels for efficient light-emitting diodes,” Nat. Nanotechnol. 11(10), 872–877 (2016).
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D. Liang, Y. Peng, Y. Fu, M. J. Shearer, J. Zhang, J. Zhai, Y. Zhang, R. J. Hamers, T. L. Andrew, and S. Jin, “Color-Pure Violet-Light-Emitting Diodes Based on Layered Lead Halide Perovskite Nanoplates,” ACS Nano 10(7), 6897–6904 (2016).
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D. Giovanni, W. K. Chong, H. A. Dewi, K. Thirumal, I. Neogi, R. Ramesh, S. Mhaisalkar, N. Mathews, and T. C. Sum, “Tunable room-temperature spin-selective optical Stark effect in solution-processed layered halide perovskites,” Sci. Adv. 2(6), e1600477 (2016).
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S. T. Ha, C. Shen, J. Zhang, and Q. H. Xiong, “Laser cooling of organic-inorganic lead halide perovskites,” Nat. Photonics 10(2), 115–121 (2016).
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C. C. Stoumpos and M. G. Kanatzidis, “Halide Perovskites: Poor Man's High-Performance Semiconductors,” Adv. Mater. 28(28), 5778–5793 (2016).
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Y. Wang, J. He, H. Chen, J. Chen, R. Zhu, P. Ma, A. Towers, Y. Lin, A. J. Gesquiere, S.-T. Wu, and Y. Dong, “Ultrastable, Highly Luminescent Organic-Inorganic Perovskite-Polymer Composite Films,” Adv. Mater. 28(48), 10710–10717 (2016).
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2015 (3)

N. J. Jeon, J. H. Noh, W. S. Yang, Y. C. Kim, S. Ryu, J. Seo, and S. I. Seok, “Compositional engineering of perovskite materials for high-performance solar cells,” Nature 517(7535), 476–480 (2015).
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L. Dou, A. B. Wong, Y. Yu, M. Lai, N. Kornienko, S. W. Eaton, A. Fu, C. G. Bischak, J. Ma, T. Ding, N. S. Ginsberg, L.-W. Wang, A. P. Alivisatos, and P. Yang, “Atomically thin two-dimensional organic-inorganic hybrid perovskites,” Science 349(6255), 1518–1521 (2015).
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X. X. Wu, M. T. Trinh, D. Niesner, H. M. Zhu, Z. Norman, J. S. Owen, O. Yaffe, B. J. Kudisch, and X. Y. Zhu, “Trap States in Lead Iodide Perovskites,” J. Am. Chem. Soc. 137(5), 2089–2096 (2015).
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2014 (5)

N. J. Jeon, J. H. Noh, Y. C. Kim, W. S. Yang, S. Ryu, and S. Il Seol, “Solvent engineering for high-performance inorganic-organic hybrid perovskite solar cells,” Nat. Mater. 13(9), 897–903 (2014).
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F. Xia, H. Wang, D. Xiao, M. Dubey, and A. Ramasubramaniam, “Two-dimensional material nanophotonics,” Nat. Photonics 8(12), 899–907 (2014).
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G. Xing, N. Mathews, S. S. Lim, N. Yantara, X. Liu, D. Sabba, M. Gratzel, S. Mhaisalkar, and T. C. Sum, “Low-temperature solution-processed wavelength-tunable perovskites for lasing,” Nat. Mater. 13(5), 476–480 (2014).
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K. G. Lim, H. B. Kim, J. Jeong, H. Kim, J. Y. Kim, and T. W. Lee, “Boosting the power conversion efficiency of perovskite solar cells using self-organized polymeric hole extraction layers with high work function,” Adv. Mater. 26(37), 6461–6466 (2014).
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X. Hu, X. Zhang, L. Liang, J. Bao, S. Li, W. Yang, and Y. Xie, “High-Performance Flexible Broadband Photodetector Based on Organolead Halide Perovskite,” Adv. Funct. Mater. 24(46), 7373–7380 (2014).
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2010 (1)

Abate, A.

A. Ummadisingu, L. Steier, J. Y. Seo, T. Matsui, A. Abate, W. Tress, and M. Gratzel, “The effect of illumination on the formation of metal halide perovskite films,” Nature 545(7653), 208–212 (2017).
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Abdi-Jalebi, M.

M. Abdi-Jalebi, Z. Andaji-Garmaroudi, S. Cacovich, C. Stavrakas, B. Philippe, J. M. Richter, M. Alsari, E. P. Booker, E. M. Hutter, A. J. Pearson, S. Lilliu, T. J. Savenije, H. Rensmo, G. Divitini, C. Ducati, R. H. Friend, and S. D. Stranks, “Maximizing and stabilizing luminescence from halide perovskites with potassium passivation,” Nature 555(7697), 497–501 (2018).
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Adjokatse, S.

H. H. Fang, J. Yang, S. X. Tao, S. Adjokatse, M. E. Kamminga, J. T. Ye, G. R. Blake, J. Even, and M. A. Loi, “Unravelling Light-Induced Degradation of Layered Perovskite Crystals and Design of Efficient Encapsulation for Improved Photostability,” Adv. Funct. Mater. 28(21), 1800305 (2018).
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Ajayan, P. M.

H. Tsai, R. Asadpour, J. C. Blancon, C. C. Stoumpos, O. Durand, J. W. Strzalka, B. Chen, R. Verduzco, P. M. Ajayan, S. Tretiak, J. Even, M. A. Alam, M. G. Kanatzidis, W. Nie, and A. D. Mohite, “Light-induced lattice expansion leads to high-efficiency perovskite solar cells,” Science 360(6384), 67–70 (2018).
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J.-C. Blancon, H. Tsai, W. Nie, C. C. Stoumpos, L. Pedesseau, C. Katan, M. Kepenekian, C. M. M. Soe, K. Appavoo, M. Y. Sfeir, S. Tretiak, P. M. Ajayan, M. G. Kanatzidis, J. Even, J. J. Crochet, and A. D. Mohite, “Extremely efficient internal exciton dissociation through edge states in layered 2D perovskites,” Science 355(6331), 1288–1292 (2017).
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Al Choueiry, A.

Alam, M. A.

H. Tsai, R. Asadpour, J. C. Blancon, C. C. Stoumpos, O. Durand, J. W. Strzalka, B. Chen, R. Verduzco, P. M. Ajayan, S. Tretiak, J. Even, M. A. Alam, M. G. Kanatzidis, W. Nie, and A. D. Mohite, “Light-induced lattice expansion leads to high-efficiency perovskite solar cells,” Science 360(6384), 67–70 (2018).
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Alivisatos, A. P.

L. Dou, A. B. Wong, Y. Yu, M. Lai, N. Kornienko, S. W. Eaton, A. Fu, C. G. Bischak, J. Ma, T. Ding, N. S. Ginsberg, L.-W. Wang, A. P. Alivisatos, and P. Yang, “Atomically thin two-dimensional organic-inorganic hybrid perovskites,” Science 349(6255), 1518–1521 (2015).
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Alsari, M.

M. Abdi-Jalebi, Z. Andaji-Garmaroudi, S. Cacovich, C. Stavrakas, B. Philippe, J. M. Richter, M. Alsari, E. P. Booker, E. M. Hutter, A. J. Pearson, S. Lilliu, T. J. Savenije, H. Rensmo, G. Divitini, C. Ducati, R. H. Friend, and S. D. Stranks, “Maximizing and stabilizing luminescence from halide perovskites with potassium passivation,” Nature 555(7697), 497–501 (2018).
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B. Zhao, S. Bai, V. Kim, R. Lamboll, R. Shivanna, F. Auras, J. M. Richter, L. Yang, L. Dai, M. Alsari, X.-J. She, L. Liang, J. Zhang, S. Lilliu, P. Gao, H. J. Snaith, J. Wang, N. C. Greenham, R. H. Friend, and D. Di, “High-efficiency perovskite-polymer bulk heterostructure light-emitting diodes,” Nat. Photonics 12(12), 783–789 (2018).
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Andaji-Garmaroudi, Z.

M. Abdi-Jalebi, Z. Andaji-Garmaroudi, S. Cacovich, C. Stavrakas, B. Philippe, J. M. Richter, M. Alsari, E. P. Booker, E. M. Hutter, A. J. Pearson, S. Lilliu, T. J. Savenije, H. Rensmo, G. Divitini, C. Ducati, R. H. Friend, and S. D. Stranks, “Maximizing and stabilizing luminescence from halide perovskites with potassium passivation,” Nature 555(7697), 497–501 (2018).
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Andrew, T. L.

D. Liang, Y. Peng, Y. Fu, M. J. Shearer, J. Zhang, J. Zhai, Y. Zhang, R. J. Hamers, T. L. Andrew, and S. Jin, “Color-Pure Violet-Light-Emitting Diodes Based on Layered Lead Halide Perovskite Nanoplates,” ACS Nano 10(7), 6897–6904 (2016).
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Appavoo, K.

J.-C. Blancon, H. Tsai, W. Nie, C. C. Stoumpos, L. Pedesseau, C. Katan, M. Kepenekian, C. M. M. Soe, K. Appavoo, M. Y. Sfeir, S. Tretiak, P. M. Ajayan, M. G. Kanatzidis, J. Even, J. J. Crochet, and A. D. Mohite, “Extremely efficient internal exciton dissociation through edge states in layered 2D perovskites,” Science 355(6331), 1288–1292 (2017).
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Asadpour, R.

H. Tsai, R. Asadpour, J. C. Blancon, C. C. Stoumpos, O. Durand, J. W. Strzalka, B. Chen, R. Verduzco, P. M. Ajayan, S. Tretiak, J. Even, M. A. Alam, M. G. Kanatzidis, W. Nie, and A. D. Mohite, “Light-induced lattice expansion leads to high-efficiency perovskite solar cells,” Science 360(6384), 67–70 (2018).
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Audebert, P.

F. Ledee, G. Trippe-Allard, H. Diab, P. Audebert, D. Garrot, J. S. Lauret, and E. Deleporte, “Fast growth of monocrystalline thin films of 2D layered hybrid perovskite,” CrystEngComm 19(19), 2598–2602 (2017).
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Auras, F.

B. Zhao, S. Bai, V. Kim, R. Lamboll, R. Shivanna, F. Auras, J. M. Richter, L. Yang, L. Dai, M. Alsari, X.-J. She, L. Liang, J. Zhang, S. Lilliu, P. Gao, H. J. Snaith, J. Wang, N. C. Greenham, R. H. Friend, and D. Di, “High-efficiency perovskite-polymer bulk heterostructure light-emitting diodes,” Nat. Photonics 12(12), 783–789 (2018).
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Bai, S.

B. Zhao, S. Bai, V. Kim, R. Lamboll, R. Shivanna, F. Auras, J. M. Richter, L. Yang, L. Dai, M. Alsari, X.-J. She, L. Liang, J. Zhang, S. Lilliu, P. Gao, H. J. Snaith, J. Wang, N. C. Greenham, R. H. Friend, and D. Di, “High-efficiency perovskite-polymer bulk heterostructure light-emitting diodes,” Nat. Photonics 12(12), 783–789 (2018).
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Bao, C.

C. Bao, Z. Chen, Y. Fang, H. Wei, Y. Deng, X. Xiao, L. Li, and J. Huang, “Low-Noise and Large-Linear-Dynamic-Range Photodetectors Based on Hybrid-Perovskite Thin-Single-Crystals,” Adv. Mater. 29(39), 1703209 (2017).
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Bao, J.

X. Hu, X. Zhang, L. Liang, J. Bao, S. Li, W. Yang, and Y. Xie, “High-Performance Flexible Broadband Photodetector Based on Organolead Halide Perovskite,” Adv. Funct. Mater. 24(46), 7373–7380 (2014).
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Beauregard, E. M.

M. Yuan, L. N. Quan, R. Comin, G. Walters, R. Sabatini, O. Voznyy, S. Hoogland, Y. Zhao, E. M. Beauregard, P. Kanjanaboos, Z. Lu, D. H. Kim, and E. H. Sargent, “Perovskite energy funnels for efficient light-emitting diodes,” Nat. Nanotechnol. 11(10), 872–877 (2016).
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Bent, S. F.

Bischak, C. G.

L. Dou, A. B. Wong, Y. Yu, M. Lai, N. Kornienko, S. W. Eaton, A. Fu, C. G. Bischak, J. Ma, T. Ding, N. S. Ginsberg, L.-W. Wang, A. P. Alivisatos, and P. Yang, “Atomically thin two-dimensional organic-inorganic hybrid perovskites,” Science 349(6255), 1518–1521 (2015).
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Blake, G. R.

H. H. Fang, J. Yang, S. X. Tao, S. Adjokatse, M. E. Kamminga, J. T. Ye, G. R. Blake, J. Even, and M. A. Loi, “Unravelling Light-Induced Degradation of Layered Perovskite Crystals and Design of Efficient Encapsulation for Improved Photostability,” Adv. Funct. Mater. 28(21), 1800305 (2018).
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Blancon, J. C.

H. Tsai, R. Asadpour, J. C. Blancon, C. C. Stoumpos, O. Durand, J. W. Strzalka, B. Chen, R. Verduzco, P. M. Ajayan, S. Tretiak, J. Even, M. A. Alam, M. G. Kanatzidis, W. Nie, and A. D. Mohite, “Light-induced lattice expansion leads to high-efficiency perovskite solar cells,” Science 360(6384), 67–70 (2018).
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Blancon, J.-C.

J.-C. Blancon, H. Tsai, W. Nie, C. C. Stoumpos, L. Pedesseau, C. Katan, M. Kepenekian, C. M. M. Soe, K. Appavoo, M. Y. Sfeir, S. Tretiak, P. M. Ajayan, M. G. Kanatzidis, J. Even, J. J. Crochet, and A. D. Mohite, “Extremely efficient internal exciton dissociation through edge states in layered 2D perovskites,” Science 355(6331), 1288–1292 (2017).
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Bloch, J.

Booker, E. P.

M. Abdi-Jalebi, Z. Andaji-Garmaroudi, S. Cacovich, C. Stavrakas, B. Philippe, J. M. Richter, M. Alsari, E. P. Booker, E. M. Hutter, A. J. Pearson, S. Lilliu, T. J. Savenije, H. Rensmo, G. Divitini, C. Ducati, R. H. Friend, and S. D. Stranks, “Maximizing and stabilizing luminescence from halide perovskites with potassium passivation,” Nature 555(7697), 497–501 (2018).
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Brehier, A.

Brenes, R.

R. Brenes, C. Eames, V. Bulovic, M. S. Islam, and S. D. Stranks, “The Impact of Atmosphere on the Local Luminescence Properties of Metal Halide Perovskite Grains,” Adv. Mater. 30(15), 1706208 (2018).
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Bu, X. H.

W. J. Wei, X. X. Jiang, L. Y. Dong, W. W. Liu, X. B. Han, Y. Qin, K. Li, W. Li, Z. S. Lin, X. H. Bu, and P. X. Lu, “Regulating Second-Harmonic Generation by van der Waals Interactions in Two-dimensional Lead Halide Perovskite Nanosheets,” J. Am. Chem. Soc. 141(23), 9134–9139 (2019).
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Bulovic, V.

R. Brenes, C. Eames, V. Bulovic, M. S. Islam, and S. D. Stranks, “The Impact of Atmosphere on the Local Luminescence Properties of Metal Halide Perovskite Grains,” Adv. Mater. 30(15), 1706208 (2018).
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Bush, K. A.

Cacovich, S.

M. Abdi-Jalebi, Z. Andaji-Garmaroudi, S. Cacovich, C. Stavrakas, B. Philippe, J. M. Richter, M. Alsari, E. P. Booker, E. M. Hutter, A. J. Pearson, S. Lilliu, T. J. Savenije, H. Rensmo, G. Divitini, C. Ducati, R. H. Friend, and S. D. Stranks, “Maximizing and stabilizing luminescence from halide perovskites with potassium passivation,” Nature 555(7697), 497–501 (2018).
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Cai, W.

D. Gui, L. Ji, A. Muhammad, W. Li, W. Cai, Y. Li, X. Li, X. Wu, and P. Lu, “Jahn-Teller Effect on Framework Flexibility of Hybrid Organic-Inorganic Perovskites,” J. Phys. Chem. Lett. 9(4), 751–755 (2018).
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Cao, F.

H. Sun, T. Lei, W. Tian, F. Cao, J. Xiong, and L. Li, “Self-Powered, Flexible, and Solution-Processable Perovskite Photodetector Based on Low-Cost Carbon Cloth,” Small 13(28), 1701042 (2017).
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Cao, Y.

M. T. Yu, C. Yi, N. N. Wang, L. D. Zhang, R. M. Zou, Y. F. Tong, H. Chen, Y. Cao, Y. R. He, Y. Wang, M. M. Xu, Y. Liu, Y. Z. Jin, W. Huang, and J. P. Wang, “Control of Barrier Width in Perovskite Multiple Quantum Wells for High Performance Green Light-Emitting Diodes,” Adv. Opt. Mater. 7(3), 1801575 (2019).
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Carpenter, J.

Cavazzini, M.

K. T. Cho, Y. Zhang, S. Orlandi, M. Cavazzini, I. Zimmermann, A. Lesch, N. Tabet, G. Pozzi, G. Grancini, and M. K. Nazeeruddin, “Water-Repellent Low-Dimensional Fluorous Perovskite as Interfacial Coating for 20% Efficient Solar Cells,” Nano Lett. 18(9), 5467–5474 (2018).
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Chehade, G.

G. Delport, G. Chehade, F. Lédée, H. Diab, C. Milesi-Brault, G. Trippé-Allard, J. Even, J.-S. Lauret, E. Deleporte, and D. Garrot, “Exciton-Exciton Annihilation in Two-Dimensional Halide Perovskites at Room Temperature,” J. Phys. Chem. Lett. 10(17), 5153–5159 (2019).
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Chen, B.

H. Tsai, R. Asadpour, J. C. Blancon, C. C. Stoumpos, O. Durand, J. W. Strzalka, B. Chen, R. Verduzco, P. M. Ajayan, S. Tretiak, J. Even, M. A. Alam, M. G. Kanatzidis, W. Nie, and A. D. Mohite, “Light-induced lattice expansion leads to high-efficiency perovskite solar cells,” Science 360(6384), 67–70 (2018).
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Chen, H.

M. T. Yu, C. Yi, N. N. Wang, L. D. Zhang, R. M. Zou, Y. F. Tong, H. Chen, Y. Cao, Y. R. He, Y. Wang, M. M. Xu, Y. Liu, Y. Z. Jin, W. Huang, and J. P. Wang, “Control of Barrier Width in Perovskite Multiple Quantum Wells for High Performance Green Light-Emitting Diodes,” Adv. Opt. Mater. 7(3), 1801575 (2019).
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Y. Wang, J. He, H. Chen, J. Chen, R. Zhu, P. Ma, A. Towers, Y. Lin, A. J. Gesquiere, S.-T. Wu, and Y. Dong, “Ultrastable, Highly Luminescent Organic-Inorganic Perovskite-Polymer Composite Films,” Adv. Mater. 28(48), 10710–10717 (2016).
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Chen, J.

Y. Wang, J. He, H. Chen, J. Chen, R. Zhu, P. Ma, A. Towers, Y. Lin, A. J. Gesquiere, S.-T. Wu, and Y. Dong, “Ultrastable, Highly Luminescent Organic-Inorganic Perovskite-Polymer Composite Films,” Adv. Mater. 28(48), 10710–10717 (2016).
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Chen, J. W.

J. W. Chen, K. Wang, H. Long, X. B. Han, H. B. Hu, W. W. Liu, B. Wang, and P. X. Lu, “Tungsten Disulfide-Gold Nanohole Hybrid Metasurfaces for Nonlinear Metalenses in the Visible Region,” Nano Lett. 18(2), 1344–1350 (2018).
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Chen, Z.

C. Bao, Z. Chen, Y. Fang, H. Wei, Y. Deng, X. Xiao, L. Li, and J. Huang, “Low-Noise and Large-Linear-Dynamic-Range Photodetectors Based on Hybrid-Perovskite Thin-Single-Crystals,” Adv. Mater. 29(39), 1703209 (2017).
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Cherukara, M.

Z. Zhang, D. Schwanz, B. Narayanan, M. Kotiuga, J. A. Dura, M. Cherukara, H. Zhou, J. W. Freeland, J. Li, R. Sutarto, F. He, C. Wu, J. Zhu, Y. Sun, K. Ramadoss, S. S. Nonnenmann, N. Yu, R. Comin, K. M. Rabe, S. Sankaranarayanan, and S. Ramanathan, “Perovskite nickelates as electric-field sensors in salt water,” Nature 553(7686), 68–72 (2018).
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Cho, K. T.

K. T. Cho, Y. Zhang, S. Orlandi, M. Cavazzini, I. Zimmermann, A. Lesch, N. Tabet, G. Pozzi, G. Grancini, and M. K. Nazeeruddin, “Water-Repellent Low-Dimensional Fluorous Perovskite as Interfacial Coating for 20% Efficient Solar Cells,” Nano Lett. 18(9), 5467–5474 (2018).
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Chong, W. K.

D. Giovanni, W. K. Chong, H. A. Dewi, K. Thirumal, I. Neogi, R. Ramesh, S. Mhaisalkar, N. Mathews, and T. C. Sum, “Tunable room-temperature spin-selective optical Stark effect in solution-processed layered halide perovskites,” Sci. Adv. 2(6), e1600477 (2016).
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Comin, R.

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J.-C. Blancon, H. Tsai, W. Nie, C. C. Stoumpos, L. Pedesseau, C. Katan, M. Kepenekian, C. M. M. Soe, K. Appavoo, M. Y. Sfeir, S. Tretiak, P. M. Ajayan, M. G. Kanatzidis, J. Even, J. J. Crochet, and A. D. Mohite, “Extremely efficient internal exciton dissociation through edge states in layered 2D perovskites,” Science 355(6331), 1288–1292 (2017).
[Crossref]

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Small (1)

H. Sun, T. Lei, W. Tian, F. Cao, J. Xiong, and L. Li, “Self-Powered, Flexible, and Solution-Processable Perovskite Photodetector Based on Low-Cost Carbon Cloth,” Small 13(28), 1701042 (2017).
[Crossref]

Other (1)

B. Wang, L. He, Y. He, Y. Zhang, R. Shao, P. Lan, and P. Lu, “All-optical measurement of high-order fractional molecular echoes by high-order harmonic generation,” eprint arXiv:1909.10514, arXiv:1909.10514 (2019).

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Figures (5)

Fig. 1.
Fig. 1. Characterization of the (PEA)2PbI4 monocrystalline films prepared in different illumination conditions. (a) Microscope images and (b) SEM images of the (PEA)2PbI4 monocrystalline films grown in the dark (Dark), and under the illumination of white light (Bright) and UV light (UV), respectively. (c) Grain size distributions of the (PEA)2PbI4 monocrystalline films.(d) Height profiles of the (PEA)2PbI4 monocrystalline films. (e) XRD patterns, and (f) the enlarged XRD peaks for the (PEA)2PbI4 monocrystalline films, respectively.
Fig. 2.
Fig. 2. The lattice expansion of the 2D perovskite induced by light illumination. (a) Plot of the increase of lattice parameters (lattice expansion) for the Bright- and UV-grown samples relative to that of the Dark-grown samples. (b) Schematic diagram for the lattice expansion. (c) Distribution of peak wavelengthes of the PL spectra under single-photon excitation for the perovskite monocrystalline films.
Fig. 3.
Fig. 3. Influence of light illumination on the PL properties of the (PEA)2PbI4 monocrystalline films. (a) Normalized PL spectra for the (PEA)2PbI4 monocrystalline films grown in the Dark, Bright, and UV conditions, respectively. (b) Single-photon excitation and (c) two-photon excitation induced PL spectra (solid curve). The gray dashed curves are the corresponding decompositions by fitting to a two-peak Lorentz model. (d) Time-resolved PL decay traces for the (PEA)2PbI4 monocrystalline films grown in the Dark, Bright, and UV conditions, respectively.
Fig. 4.
Fig. 4. Controllable crystal quality and PL performance of the (PEA)2PbI4 monocrystalline films through light illumination. (a) Enlarged XRD patterns and (b) PL spectra of the (PEA)2PbI4 monocrystalline films grown under UV-light illumination, with various intensity. The insets show the corresponding microscope images.
Fig. 5.
Fig. 5. Optoelectronic characteristics of the photoconductive device fabricated based on the (PEA)2PbI4 monocrystalline films grown under UV condition [(a)–(f)], and dark condition [(g)–(l)]. (a)(g) I-V curves of the device in dark and under a 518-nm light with different powers. The inset shows the optical image of the as-fabricated device. The scale bar is 100 µm. (b)(h) The spectral response of the device under different biases. (c)(i) The optical switch characteristics of the device under a switched-on/off 518-nm light irradiation with different powers at the bias of –9 V. (d)(j) Transient photocurrent response under a 518-nm light illumination at the bias of –9 V. (e)(k) Normalized frequency response of the device at the bias of –9 V. The 3-dB bandwidth is 8.5 Hz. (f)(l) Detectivity (D*) spectrum of the device at the bias of −9 V. The insets show the noise power density (Sn) spectrum of the device.

Tables (1)

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Table 1. XRD peaks and the corresponding lattice parameters extracted from the XRD patterns for the 2D perovskite monocrystalline films prepared under different illumination conditions.

Equations (1)

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D =   ( A Δ f ) 1 / 2 / NEP

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