Abstract

We report the linear and nonlinear optical (NLO) properties of a polar crystal Cs2TeW3O12 (CTW). The second-order NLO coefficients were determined by Maker Fringe (MF) techniques for the first time. CTW belong to hexagonal system with point group P63, the two independent NLO coefficients of d32 and d33 were determined to be 6.2 and 4.3 pm/V, respectively. CTW can realize phase-matching (PM) and in the direction of θ = 39.6° the effective NLO coefficient is 4.0 pm/V at 1064 nm. To illustrate the good NLO properties of CTW, the distortions of polyhedron structures were also discussed in detail.

© 2016 Optical Society of America

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References

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    [Crossref]
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    [Crossref]
  36. J. J. Zhang, Z. H. Zhang, Y. X. Sun, C. Q. Zhang, and X. T. Tao, “Anisotropic thermal properties of the polar crystal Cs2TeMo3O12,” J. Solid State Chem. 195, 120–124 (2012).
    [Crossref]
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    [Crossref]

2015 (1)

P. Zhao, H. J. Cong, X. X. Tian, Y. X. Sun, C. Q. Zhang, S. Q. Xia, Z. L. Gao, and X. T. Tao, “Top-Seeded Solution Growth, Structure, Morphology, and Functional Properties of a New Polar Crystal – Cs2TeW3O12,” Cryst. Growth Des. 15(9), 4484–4489 (2015).
[Crossref]

2014 (1)

X. X. Feng, J. J. Zhang, Z. L. Gao, S. J. Zhang, Y. X. Sun, and X. T. Tao, “Investigation of the second-order nonlinear optical properties of Cs2TeMo3O12 single crystal,” Appl. Phys. Lett. 104(8), 081912 (2014).
[Crossref]

2012 (7)

Q. X. Yu, Z. L. Gao, S. J. Zhang, W. G. Zhang, S. P. Wang, and X. T. Tao, “Second order nonlinear properties of monoclinic single crystal BaTeMo2O9,” J. Appl. Phys. 111(1), 013506 (2012).
[Crossref]

J. Yeon, S.-H. Kim, S. D. Nguyen, H. Lee, and P. S. Halasyamani, “Two New Noncentrosymmetric (NCS) Polar Oxides: Syntheses, Characterization, and Structure-Property Relationships in BaMTe2O7 (M = Mg2+ or Zn2+),” Inorg. Chem. 51(4), 2662–2668 (2012).
[Crossref] [PubMed]

S. D. Nguyen and P. S. Halasyamani, “Synthesis, Structure, and Characterization of New Li+-d0-Lone-Pair-Oxides: Noncentrosymmetric Polar Li6(Mo2O5)3(SeO3)6 and Centrosymmetric Li2(MO3)(TeO3) (M = Mo6+ or W6+),” Inorg. Chem. 51(17), 9529–9538 (2012).
[Crossref] [PubMed]

J. J. Zhang, Z. H. Zhang, Y. X. Sun, C. Q. Zhang, S. J. Zhang, Y. Liu, and X. T. Tao, “MgTeMoO6: A neutral layered material showing strong second-harmonic generation,” J. Mater. Chem. 22(19), 9921–9927 (2012).
[Crossref]

I. Georgescu, “Lasers: Symphony of lights,” Nat. Phys. 8(9), 639 (2012).
[Crossref]

C. Skrobol, I. Ahmad, S. Klingebiel, C. Wandt, S. A. Trushin, Z. Major, F. Krausz, and S. Karsch, “Broadband amplification by picosecond OPCPA in DKDP pumped at 515 nm,” Opt. Express 20(4), 4619–4629 (2012).
[Crossref] [PubMed]

J. J. Zhang, Z. H. Zhang, Y. X. Sun, C. Q. Zhang, and X. T. Tao, “Anisotropic thermal properties of the polar crystal Cs2TeMo3O12,” J. Solid State Chem. 195, 120–124 (2012).
[Crossref]

2011 (4)

S. D. Nguyen, J. Yeon, S.-H. Kim, and P. S. Halasyamani, “BiO(IO3): A New Polar Iodate that Exhibits An Aurivillius-Type (Bi2O2)2+ Layer and a Large SHG Response,” J. Am. Chem. Soc. 133(32), 12422–12425 (2011).
[Crossref] [PubMed]

J. J. Zhang, X. T. Tao, Y. X. Sun, Z. H. Zhang, C. Q. Zhang, Z. L. Gao, H. B. Xia, and S. Q. Xia, “Top-Seeded Solution Growth, Morphology, and Properties of a Polar Crystal Cs2TeMo3O12,” Cryst. Growth Des. 11(5), 1863–1868 (2011).
[Crossref]

J. J. Zhang, Z. H. Zhang, W. G. Zhang, Q. X. Zheng, Y. X. Sun, C. Q. Zhang, and X. Tao, “Polymorphism of BaTeMo2O9: A New Polar Polymorph and the Phase Transformation,” Chem. Mater. 23(16), 3752–3761 (2011).
[Crossref]

S. D. Nguyen, S.-H. Kim, and P. S. Halasyamani, “Synthesis, Characterization, and Structure-Property Relationships in Two New Polar Oxides: Zn2(MoO4)(SeO3) and Zn2(MoO4)(TeO3),” Inorg. Chem. 50(11), 5215–5222 (2011).
[Crossref] [PubMed]

2010 (2)

W. G. Zhang, F. Li, S.-H. Kim, and P. S. Halasyamani, “Top-Seeded Solution Crystal Growth and Functional Properties of a Polar Material–Na2TeW2O9,” Cryst. Growth Des. 10(9), 4091–4095 (2010).
[Crossref]

N. Ye, C. Y. Tu, X. F. Long, and M. C. Hong, “Recent Advances in crystal growth in china: laser, nonlinear optical, and ferroelectric crystals,” Cryst. Growth Des. 10(11), 4672–4681 (2010).
[Crossref]

2009 (3)

C. T. Chen, G. L. Wang, X. Y. Wang, and Z. Y. Xu, “Deep-UV nonlinear optical crystal KBe2BO3F2– discovery, growth, optical properties and applications,” Appl. Phys. B 97(1), 9–25 (2009).
[Crossref]

T. Kanai, X. Wang, S. Adachi, S. Watanabe, and C. Chen, “Watt-level tunable deep ultraviolet light source by a KBBF prism-coupled device,” Opt. Express 17(10), 8696–8703 (2009).
[Crossref] [PubMed]

C. F. Sun, C. L. Hu, X. Xu, J. B. Ling, T. Hu, F. Kong, X. F. Long, and J. G. Mao, “BaNbO(IO3)5: A New Polar Material with a Very Large SHG Response,” J. Am. Chem. Soc. 131(27), 9486–9487 (2009).
[Crossref] [PubMed]

2008 (2)

W. G. Zhang, X. T. Tao, C. Q. Zhang, Z. L. Gao, Y. Z. Zhang, W. T. Yu, X. F. Cheng, X. S. Li, and M. H. Jiang, “Bulk Growth and Characterization of a Novel Nonlinear Optical Crystal BaTeMo2O9,” Cryst. Growth Des. 8(1), 304–307 (2008).
[Crossref]

B. Zhao, Y. Jiang, K. Sueda, N. Miyanaga, and T. Kobayashi, “Ultrabroadband noncollinear optical parametric amplification with LBO crystal,” Opt. Express 16(23), 18863–18868 (2008).
[Crossref] [PubMed]

2007 (2)

2006 (2)

H. Peng, W. Hou, Y. Chen, D. Cui, Z. Xu, C. Chen, F. Fan, and Y. Zhu, “28W red light output at 659.5nm by intracavity frequency doubling of a Nd:YAG laser using LBO,” Opt. Express 14(9), 3961–3967 (2006).
[Crossref] [PubMed]

E. O. Chi, K. M. Ok, Y. Porter, and P. S. Halasyamani, “Na2Te3Mo3O16: A New Molybdenum Tellurite with Second-Harmonic Generating and Pyroelectric Properties,” Chem. Mater. 18(8), 2070–2074 (2006).
[Crossref]

2004 (1)

P. Shiv Halasyamani, “Asymmetric Cation Coordination in Oxide Materials: Influence of Lone-Pair Cations on the Intra-octahedral Distortion in d0 Transition Metals,” Chem. Mater. 16(19), 3586–3592 (2004).
[Crossref]

2003 (3)

2002 (1)

J. Goodey, J. Broussard, and P. S. Halasyamani, “Synthesis, Structure, and Characterization of a New Second-Harmonic-Generating Tellurite: Na2TeW2O9,” Chem. Mater. 14(7), 3174–3180 (2002).
[Crossref]

1998 (1)

P. S. Halasyamani and K. R. Poeppelmeier, “Noncentrosymmetric oxides,” Chem. Mater. 10(10), 2753–2769 (1998).
[Crossref]

1993 (1)

1992 (1)

D. A. Roberts, “Simplified characterization of uniaxial and biaxial nonlinear optical crystals: a plea for standardization of nomenclature and conventions,” IEEE J. Quantum Electron. 28(10), 2057–2074 (1992).
[Crossref]

1991 (1)

1989 (1)

S. X. Dou, M. H. Jiang, Z. S. Shao, and X. T. Tao, “Maker fringes in biaxial crystals and the nonlinear optical coefficients of thiosemicarbazide cadmium chloride monohydrate,” Appl. Phys. Lett. 54(12), 1101–1103 (1989).
[Crossref]

1987 (1)

D. Eimerl, “Electro-optic, linear and nonlinear optical properties of KDP and its isomorphs,” Ferroelectrics 72(1), 95–139 (1987).
[Crossref]

1962 (1)

D. A. Kleinman, “Nonlinear dielectric polarization in optical media,” Phys. Rev. 126(6), 1977–1979 (1962).
[Crossref]

Adachi, S.

Ahmad, I.

Broussard, J.

J. Goodey, J. Broussard, and P. S. Halasyamani, “Synthesis, Structure, and Characterization of a New Second-Harmonic-Generating Tellurite: Na2TeW2O9,” Chem. Mater. 14(7), 3174–3180 (2002).
[Crossref]

Chen, C.

Chen, C. T.

C. T. Chen, G. L. Wang, X. Y. Wang, and Z. Y. Xu, “Deep-UV nonlinear optical crystal KBe2BO3F2– discovery, growth, optical properties and applications,” Appl. Phys. B 97(1), 9–25 (2009).
[Crossref]

X. Zhang, X. A. Wang, G. L. Wang, Y. C. Wu, Y. Zhu, and C. T. Chen, “Determination of the nonlinear optical coefficients of the LixCs(1 – x)B3O5 crystals,” J. Opt. Soc. Am. B 24(11), 2877–2882 (2007).
[Crossref]

Chen, Y.

Cheng, X. F.

W. G. Zhang, X. T. Tao, C. Q. Zhang, Z. L. Gao, Y. Z. Zhang, W. T. Yu, X. F. Cheng, X. S. Li, and M. H. Jiang, “Bulk Growth and Characterization of a Novel Nonlinear Optical Crystal BaTeMo2O9,” Cryst. Growth Des. 8(1), 304–307 (2008).
[Crossref]

Chi, E. O.

E. O. Chi, K. M. Ok, Y. Porter, and P. S. Halasyamani, “Na2Te3Mo3O16: A New Molybdenum Tellurite with Second-Harmonic Generating and Pyroelectric Properties,” Chem. Mater. 18(8), 2070–2074 (2006).
[Crossref]

Cong, H. J.

P. Zhao, H. J. Cong, X. X. Tian, Y. X. Sun, C. Q. Zhang, S. Q. Xia, Z. L. Gao, and X. T. Tao, “Top-Seeded Solution Growth, Structure, Morphology, and Functional Properties of a New Polar Crystal – Cs2TeW3O12,” Cryst. Growth Des. 15(9), 4484–4489 (2015).
[Crossref]

Cui, D.

Dou, S. X.

S. X. Dou, M. H. Jiang, Z. S. Shao, and X. T. Tao, “Maker fringes in biaxial crystals and the nonlinear optical coefficients of thiosemicarbazide cadmium chloride monohydrate,” Appl. Phys. Lett. 54(12), 1101–1103 (1989).
[Crossref]

Eimerl, D.

D. Eimerl, “Electro-optic, linear and nonlinear optical properties of KDP and its isomorphs,” Ferroelectrics 72(1), 95–139 (1987).
[Crossref]

Ellingson, R. J.

Fan, F.

Feng, X. X.

X. X. Feng, J. J. Zhang, Z. L. Gao, S. J. Zhang, Y. X. Sun, and X. T. Tao, “Investigation of the second-order nonlinear optical properties of Cs2TeMo3O12 single crystal,” Appl. Phys. Lett. 104(8), 081912 (2014).
[Crossref]

Gao, Z. L.

P. Zhao, H. J. Cong, X. X. Tian, Y. X. Sun, C. Q. Zhang, S. Q. Xia, Z. L. Gao, and X. T. Tao, “Top-Seeded Solution Growth, Structure, Morphology, and Functional Properties of a New Polar Crystal – Cs2TeW3O12,” Cryst. Growth Des. 15(9), 4484–4489 (2015).
[Crossref]

X. X. Feng, J. J. Zhang, Z. L. Gao, S. J. Zhang, Y. X. Sun, and X. T. Tao, “Investigation of the second-order nonlinear optical properties of Cs2TeMo3O12 single crystal,” Appl. Phys. Lett. 104(8), 081912 (2014).
[Crossref]

Q. X. Yu, Z. L. Gao, S. J. Zhang, W. G. Zhang, S. P. Wang, and X. T. Tao, “Second order nonlinear properties of monoclinic single crystal BaTeMo2O9,” J. Appl. Phys. 111(1), 013506 (2012).
[Crossref]

J. J. Zhang, X. T. Tao, Y. X. Sun, Z. H. Zhang, C. Q. Zhang, Z. L. Gao, H. B. Xia, and S. Q. Xia, “Top-Seeded Solution Growth, Morphology, and Properties of a Polar Crystal Cs2TeMo3O12,” Cryst. Growth Des. 11(5), 1863–1868 (2011).
[Crossref]

W. G. Zhang, X. T. Tao, C. Q. Zhang, Z. L. Gao, Y. Z. Zhang, W. T. Yu, X. F. Cheng, X. S. Li, and M. H. Jiang, “Bulk Growth and Characterization of a Novel Nonlinear Optical Crystal BaTeMo2O9,” Cryst. Growth Des. 8(1), 304–307 (2008).
[Crossref]

Georgescu, I.

I. Georgescu, “Lasers: Symphony of lights,” Nat. Phys. 8(9), 639 (2012).
[Crossref]

Goodey, J.

J. Goodey, J. Broussard, and P. S. Halasyamani, “Synthesis, Structure, and Characterization of a New Second-Harmonic-Generating Tellurite: Na2TeW2O9,” Chem. Mater. 14(7), 3174–3180 (2002).
[Crossref]

Halasyamani, P. S.

J. Yeon, S.-H. Kim, S. D. Nguyen, H. Lee, and P. S. Halasyamani, “Two New Noncentrosymmetric (NCS) Polar Oxides: Syntheses, Characterization, and Structure-Property Relationships in BaMTe2O7 (M = Mg2+ or Zn2+),” Inorg. Chem. 51(4), 2662–2668 (2012).
[Crossref] [PubMed]

S. D. Nguyen and P. S. Halasyamani, “Synthesis, Structure, and Characterization of New Li+-d0-Lone-Pair-Oxides: Noncentrosymmetric Polar Li6(Mo2O5)3(SeO3)6 and Centrosymmetric Li2(MO3)(TeO3) (M = Mo6+ or W6+),” Inorg. Chem. 51(17), 9529–9538 (2012).
[Crossref] [PubMed]

S. D. Nguyen, S.-H. Kim, and P. S. Halasyamani, “Synthesis, Characterization, and Structure-Property Relationships in Two New Polar Oxides: Zn2(MoO4)(SeO3) and Zn2(MoO4)(TeO3),” Inorg. Chem. 50(11), 5215–5222 (2011).
[Crossref] [PubMed]

S. D. Nguyen, J. Yeon, S.-H. Kim, and P. S. Halasyamani, “BiO(IO3): A New Polar Iodate that Exhibits An Aurivillius-Type (Bi2O2)2+ Layer and a Large SHG Response,” J. Am. Chem. Soc. 133(32), 12422–12425 (2011).
[Crossref] [PubMed]

W. G. Zhang, F. Li, S.-H. Kim, and P. S. Halasyamani, “Top-Seeded Solution Crystal Growth and Functional Properties of a Polar Material–Na2TeW2O9,” Cryst. Growth Des. 10(9), 4091–4095 (2010).
[Crossref]

E. O. Chi, K. M. Ok, Y. Porter, and P. S. Halasyamani, “Na2Te3Mo3O16: A New Molybdenum Tellurite with Second-Harmonic Generating and Pyroelectric Properties,” Chem. Mater. 18(8), 2070–2074 (2006).
[Crossref]

H. S. Ra, K. M. Ok, and P. S. Halasyamani, “Combining Second-Order Jahn-Teller Distorted Cations to Create Highly Efficient SHG Materials: Synthesis, Characterization, and NLO Properties of BaTeM2O9 (M = Mo6+ or W6+),” J. Am. Chem. Soc. 125(26), 7764–7765 (2003).
[Crossref] [PubMed]

J. Goodey, J. Broussard, and P. S. Halasyamani, “Synthesis, Structure, and Characterization of a New Second-Harmonic-Generating Tellurite: Na2TeW2O9,” Chem. Mater. 14(7), 3174–3180 (2002).
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P. S. Halasyamani and K. R. Poeppelmeier, “Noncentrosymmetric oxides,” Chem. Mater. 10(10), 2753–2769 (1998).
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N. Ye, C. Y. Tu, X. F. Long, and M. C. Hong, “Recent Advances in crystal growth in china: laser, nonlinear optical, and ferroelectric crystals,” Cryst. Growth Des. 10(11), 4672–4681 (2010).
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Hu, C. L.

C. F. Sun, C. L. Hu, X. Xu, J. B. Ling, T. Hu, F. Kong, X. F. Long, and J. G. Mao, “BaNbO(IO3)5: A New Polar Material with a Very Large SHG Response,” J. Am. Chem. Soc. 131(27), 9486–9487 (2009).
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Hu, T.

C. F. Sun, C. L. Hu, X. Xu, J. B. Ling, T. Hu, F. Kong, X. F. Long, and J. G. Mao, “BaNbO(IO3)5: A New Polar Material with a Very Large SHG Response,” J. Am. Chem. Soc. 131(27), 9486–9487 (2009).
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Jiang, M. H.

W. G. Zhang, X. T. Tao, C. Q. Zhang, Z. L. Gao, Y. Z. Zhang, W. T. Yu, X. F. Cheng, X. S. Li, and M. H. Jiang, “Bulk Growth and Characterization of a Novel Nonlinear Optical Crystal BaTeMo2O9,” Cryst. Growth Des. 8(1), 304–307 (2008).
[Crossref]

S. X. Dou, M. H. Jiang, Z. S. Shao, and X. T. Tao, “Maker fringes in biaxial crystals and the nonlinear optical coefficients of thiosemicarbazide cadmium chloride monohydrate,” Appl. Phys. Lett. 54(12), 1101–1103 (1989).
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S. D. Nguyen, J. Yeon, S.-H. Kim, and P. S. Halasyamani, “BiO(IO3): A New Polar Iodate that Exhibits An Aurivillius-Type (Bi2O2)2+ Layer and a Large SHG Response,” J. Am. Chem. Soc. 133(32), 12422–12425 (2011).
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S. D. Nguyen, S.-H. Kim, and P. S. Halasyamani, “Synthesis, Characterization, and Structure-Property Relationships in Two New Polar Oxides: Zn2(MoO4)(SeO3) and Zn2(MoO4)(TeO3),” Inorg. Chem. 50(11), 5215–5222 (2011).
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W. G. Zhang, F. Li, S.-H. Kim, and P. S. Halasyamani, “Top-Seeded Solution Crystal Growth and Functional Properties of a Polar Material–Na2TeW2O9,” Cryst. Growth Des. 10(9), 4091–4095 (2010).
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Krausz, F.

Lee, C.-K.

Lee, H.

J. Yeon, S.-H. Kim, S. D. Nguyen, H. Lee, and P. S. Halasyamani, “Two New Noncentrosymmetric (NCS) Polar Oxides: Syntheses, Characterization, and Structure-Property Relationships in BaMTe2O7 (M = Mg2+ or Zn2+),” Inorg. Chem. 51(4), 2662–2668 (2012).
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W. G. Zhang, F. Li, S.-H. Kim, and P. S. Halasyamani, “Top-Seeded Solution Crystal Growth and Functional Properties of a Polar Material–Na2TeW2O9,” Cryst. Growth Des. 10(9), 4091–4095 (2010).
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W. G. Zhang, X. T. Tao, C. Q. Zhang, Z. L. Gao, Y. Z. Zhang, W. T. Yu, X. F. Cheng, X. S. Li, and M. H. Jiang, “Bulk Growth and Characterization of a Novel Nonlinear Optical Crystal BaTeMo2O9,” Cryst. Growth Des. 8(1), 304–307 (2008).
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C. F. Sun, C. L. Hu, X. Xu, J. B. Ling, T. Hu, F. Kong, X. F. Long, and J. G. Mao, “BaNbO(IO3)5: A New Polar Material with a Very Large SHG Response,” J. Am. Chem. Soc. 131(27), 9486–9487 (2009).
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J. J. Zhang, Z. H. Zhang, Y. X. Sun, C. Q. Zhang, S. J. Zhang, Y. Liu, and X. T. Tao, “MgTeMoO6: A neutral layered material showing strong second-harmonic generation,” J. Mater. Chem. 22(19), 9921–9927 (2012).
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N. Ye, C. Y. Tu, X. F. Long, and M. C. Hong, “Recent Advances in crystal growth in china: laser, nonlinear optical, and ferroelectric crystals,” Cryst. Growth Des. 10(11), 4672–4681 (2010).
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C. F. Sun, C. L. Hu, X. Xu, J. B. Ling, T. Hu, F. Kong, X. F. Long, and J. G. Mao, “BaNbO(IO3)5: A New Polar Material with a Very Large SHG Response,” J. Am. Chem. Soc. 131(27), 9486–9487 (2009).
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Mao, J. G.

C. F. Sun, C. L. Hu, X. Xu, J. B. Ling, T. Hu, F. Kong, X. F. Long, and J. G. Mao, “BaNbO(IO3)5: A New Polar Material with a Very Large SHG Response,” J. Am. Chem. Soc. 131(27), 9486–9487 (2009).
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Nguyen, S. D.

J. Yeon, S.-H. Kim, S. D. Nguyen, H. Lee, and P. S. Halasyamani, “Two New Noncentrosymmetric (NCS) Polar Oxides: Syntheses, Characterization, and Structure-Property Relationships in BaMTe2O7 (M = Mg2+ or Zn2+),” Inorg. Chem. 51(4), 2662–2668 (2012).
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S. D. Nguyen and P. S. Halasyamani, “Synthesis, Structure, and Characterization of New Li+-d0-Lone-Pair-Oxides: Noncentrosymmetric Polar Li6(Mo2O5)3(SeO3)6 and Centrosymmetric Li2(MO3)(TeO3) (M = Mo6+ or W6+),” Inorg. Chem. 51(17), 9529–9538 (2012).
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S. D. Nguyen, S.-H. Kim, and P. S. Halasyamani, “Synthesis, Characterization, and Structure-Property Relationships in Two New Polar Oxides: Zn2(MoO4)(SeO3) and Zn2(MoO4)(TeO3),” Inorg. Chem. 50(11), 5215–5222 (2011).
[Crossref] [PubMed]

S. D. Nguyen, J. Yeon, S.-H. Kim, and P. S. Halasyamani, “BiO(IO3): A New Polar Iodate that Exhibits An Aurivillius-Type (Bi2O2)2+ Layer and a Large SHG Response,” J. Am. Chem. Soc. 133(32), 12422–12425 (2011).
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E. O. Chi, K. M. Ok, Y. Porter, and P. S. Halasyamani, “Na2Te3Mo3O16: A New Molybdenum Tellurite with Second-Harmonic Generating and Pyroelectric Properties,” Chem. Mater. 18(8), 2070–2074 (2006).
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H. S. Ra, K. M. Ok, and P. S. Halasyamani, “Combining Second-Order Jahn-Teller Distorted Cations to Create Highly Efficient SHG Materials: Synthesis, Characterization, and NLO Properties of BaTeM2O9 (M = Mo6+ or W6+),” J. Am. Chem. Soc. 125(26), 7764–7765 (2003).
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Peng, H.

Poeppelmeier, K. R.

P. S. Halasyamani and K. R. Poeppelmeier, “Noncentrosymmetric oxides,” Chem. Mater. 10(10), 2753–2769 (1998).
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E. O. Chi, K. M. Ok, Y. Porter, and P. S. Halasyamani, “Na2Te3Mo3O16: A New Molybdenum Tellurite with Second-Harmonic Generating and Pyroelectric Properties,” Chem. Mater. 18(8), 2070–2074 (2006).
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H. S. Ra, K. M. Ok, and P. S. Halasyamani, “Combining Second-Order Jahn-Teller Distorted Cations to Create Highly Efficient SHG Materials: Synthesis, Characterization, and NLO Properties of BaTeM2O9 (M = Mo6+ or W6+),” J. Am. Chem. Soc. 125(26), 7764–7765 (2003).
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Shao, Z. S.

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Sueda, K.

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C. F. Sun, C. L. Hu, X. Xu, J. B. Ling, T. Hu, F. Kong, X. F. Long, and J. G. Mao, “BaNbO(IO3)5: A New Polar Material with a Very Large SHG Response,” J. Am. Chem. Soc. 131(27), 9486–9487 (2009).
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Sun, Y. X.

P. Zhao, H. J. Cong, X. X. Tian, Y. X. Sun, C. Q. Zhang, S. Q. Xia, Z. L. Gao, and X. T. Tao, “Top-Seeded Solution Growth, Structure, Morphology, and Functional Properties of a New Polar Crystal – Cs2TeW3O12,” Cryst. Growth Des. 15(9), 4484–4489 (2015).
[Crossref]

X. X. Feng, J. J. Zhang, Z. L. Gao, S. J. Zhang, Y. X. Sun, and X. T. Tao, “Investigation of the second-order nonlinear optical properties of Cs2TeMo3O12 single crystal,” Appl. Phys. Lett. 104(8), 081912 (2014).
[Crossref]

J. J. Zhang, Z. H. Zhang, Y. X. Sun, C. Q. Zhang, and X. T. Tao, “Anisotropic thermal properties of the polar crystal Cs2TeMo3O12,” J. Solid State Chem. 195, 120–124 (2012).
[Crossref]

J. J. Zhang, Z. H. Zhang, Y. X. Sun, C. Q. Zhang, S. J. Zhang, Y. Liu, and X. T. Tao, “MgTeMoO6: A neutral layered material showing strong second-harmonic generation,” J. Mater. Chem. 22(19), 9921–9927 (2012).
[Crossref]

J. J. Zhang, Z. H. Zhang, W. G. Zhang, Q. X. Zheng, Y. X. Sun, C. Q. Zhang, and X. Tao, “Polymorphism of BaTeMo2O9: A New Polar Polymorph and the Phase Transformation,” Chem. Mater. 23(16), 3752–3761 (2011).
[Crossref]

J. J. Zhang, X. T. Tao, Y. X. Sun, Z. H. Zhang, C. Q. Zhang, Z. L. Gao, H. B. Xia, and S. Q. Xia, “Top-Seeded Solution Growth, Morphology, and Properties of a Polar Crystal Cs2TeMo3O12,” Cryst. Growth Des. 11(5), 1863–1868 (2011).
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Tao, X.

J. J. Zhang, Z. H. Zhang, W. G. Zhang, Q. X. Zheng, Y. X. Sun, C. Q. Zhang, and X. Tao, “Polymorphism of BaTeMo2O9: A New Polar Polymorph and the Phase Transformation,” Chem. Mater. 23(16), 3752–3761 (2011).
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P. Zhao, H. J. Cong, X. X. Tian, Y. X. Sun, C. Q. Zhang, S. Q. Xia, Z. L. Gao, and X. T. Tao, “Top-Seeded Solution Growth, Structure, Morphology, and Functional Properties of a New Polar Crystal – Cs2TeW3O12,” Cryst. Growth Des. 15(9), 4484–4489 (2015).
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X. X. Feng, J. J. Zhang, Z. L. Gao, S. J. Zhang, Y. X. Sun, and X. T. Tao, “Investigation of the second-order nonlinear optical properties of Cs2TeMo3O12 single crystal,” Appl. Phys. Lett. 104(8), 081912 (2014).
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Q. X. Yu, Z. L. Gao, S. J. Zhang, W. G. Zhang, S. P. Wang, and X. T. Tao, “Second order nonlinear properties of monoclinic single crystal BaTeMo2O9,” J. Appl. Phys. 111(1), 013506 (2012).
[Crossref]

J. J. Zhang, Z. H. Zhang, Y. X. Sun, C. Q. Zhang, and X. T. Tao, “Anisotropic thermal properties of the polar crystal Cs2TeMo3O12,” J. Solid State Chem. 195, 120–124 (2012).
[Crossref]

J. J. Zhang, Z. H. Zhang, Y. X. Sun, C. Q. Zhang, S. J. Zhang, Y. Liu, and X. T. Tao, “MgTeMoO6: A neutral layered material showing strong second-harmonic generation,” J. Mater. Chem. 22(19), 9921–9927 (2012).
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J. J. Zhang, X. T. Tao, Y. X. Sun, Z. H. Zhang, C. Q. Zhang, Z. L. Gao, H. B. Xia, and S. Q. Xia, “Top-Seeded Solution Growth, Morphology, and Properties of a Polar Crystal Cs2TeMo3O12,” Cryst. Growth Des. 11(5), 1863–1868 (2011).
[Crossref]

W. G. Zhang, X. T. Tao, C. Q. Zhang, Z. L. Gao, Y. Z. Zhang, W. T. Yu, X. F. Cheng, X. S. Li, and M. H. Jiang, “Bulk Growth and Characterization of a Novel Nonlinear Optical Crystal BaTeMo2O9,” Cryst. Growth Des. 8(1), 304–307 (2008).
[Crossref]

S. X. Dou, M. H. Jiang, Z. S. Shao, and X. T. Tao, “Maker fringes in biaxial crystals and the nonlinear optical coefficients of thiosemicarbazide cadmium chloride monohydrate,” Appl. Phys. Lett. 54(12), 1101–1103 (1989).
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P. Zhao, H. J. Cong, X. X. Tian, Y. X. Sun, C. Q. Zhang, S. Q. Xia, Z. L. Gao, and X. T. Tao, “Top-Seeded Solution Growth, Structure, Morphology, and Functional Properties of a New Polar Crystal – Cs2TeW3O12,” Cryst. Growth Des. 15(9), 4484–4489 (2015).
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N. Ye, C. Y. Tu, X. F. Long, and M. C. Hong, “Recent Advances in crystal growth in china: laser, nonlinear optical, and ferroelectric crystals,” Cryst. Growth Des. 10(11), 4672–4681 (2010).
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Wang, G. L.

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Q. X. Yu, Z. L. Gao, S. J. Zhang, W. G. Zhang, S. P. Wang, and X. T. Tao, “Second order nonlinear properties of monoclinic single crystal BaTeMo2O9,” J. Appl. Phys. 111(1), 013506 (2012).
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Wang, X. A.

Wang, X. Y.

C. T. Chen, G. L. Wang, X. Y. Wang, and Z. Y. Xu, “Deep-UV nonlinear optical crystal KBe2BO3F2– discovery, growth, optical properties and applications,” Appl. Phys. B 97(1), 9–25 (2009).
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Wu, B.

Wu, Y. C.

Xia, H. B.

J. J. Zhang, X. T. Tao, Y. X. Sun, Z. H. Zhang, C. Q. Zhang, Z. L. Gao, H. B. Xia, and S. Q. Xia, “Top-Seeded Solution Growth, Morphology, and Properties of a Polar Crystal Cs2TeMo3O12,” Cryst. Growth Des. 11(5), 1863–1868 (2011).
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Xia, S. Q.

P. Zhao, H. J. Cong, X. X. Tian, Y. X. Sun, C. Q. Zhang, S. Q. Xia, Z. L. Gao, and X. T. Tao, “Top-Seeded Solution Growth, Structure, Morphology, and Functional Properties of a New Polar Crystal – Cs2TeW3O12,” Cryst. Growth Des. 15(9), 4484–4489 (2015).
[Crossref]

J. J. Zhang, X. T. Tao, Y. X. Sun, Z. H. Zhang, C. Q. Zhang, Z. L. Gao, H. B. Xia, and S. Q. Xia, “Top-Seeded Solution Growth, Morphology, and Properties of a Polar Crystal Cs2TeMo3O12,” Cryst. Growth Des. 11(5), 1863–1868 (2011).
[Crossref]

Xie, F.

Xu, X.

C. F. Sun, C. L. Hu, X. Xu, J. B. Ling, T. Hu, F. Kong, X. F. Long, and J. G. Mao, “BaNbO(IO3)5: A New Polar Material with a Very Large SHG Response,” J. Am. Chem. Soc. 131(27), 9486–9487 (2009).
[Crossref] [PubMed]

Xu, Z.

Xu, Z. Y.

C. T. Chen, G. L. Wang, X. Y. Wang, and Z. Y. Xu, “Deep-UV nonlinear optical crystal KBe2BO3F2– discovery, growth, optical properties and applications,” Appl. Phys. B 97(1), 9–25 (2009).
[Crossref]

Ye, N.

N. Ye, C. Y. Tu, X. F. Long, and M. C. Hong, “Recent Advances in crystal growth in china: laser, nonlinear optical, and ferroelectric crystals,” Cryst. Growth Des. 10(11), 4672–4681 (2010).
[Crossref]

Yeon, J.

J. Yeon, S.-H. Kim, S. D. Nguyen, H. Lee, and P. S. Halasyamani, “Two New Noncentrosymmetric (NCS) Polar Oxides: Syntheses, Characterization, and Structure-Property Relationships in BaMTe2O7 (M = Mg2+ or Zn2+),” Inorg. Chem. 51(4), 2662–2668 (2012).
[Crossref] [PubMed]

S. D. Nguyen, J. Yeon, S.-H. Kim, and P. S. Halasyamani, “BiO(IO3): A New Polar Iodate that Exhibits An Aurivillius-Type (Bi2O2)2+ Layer and a Large SHG Response,” J. Am. Chem. Soc. 133(32), 12422–12425 (2011).
[Crossref] [PubMed]

You, G.

Yu, Q. X.

Q. X. Yu, Z. L. Gao, S. J. Zhang, W. G. Zhang, S. P. Wang, and X. T. Tao, “Second order nonlinear properties of monoclinic single crystal BaTeMo2O9,” J. Appl. Phys. 111(1), 013506 (2012).
[Crossref]

Yu, W. T.

W. G. Zhang, X. T. Tao, C. Q. Zhang, Z. L. Gao, Y. Z. Zhang, W. T. Yu, X. F. Cheng, X. S. Li, and M. H. Jiang, “Bulk Growth and Characterization of a Novel Nonlinear Optical Crystal BaTeMo2O9,” Cryst. Growth Des. 8(1), 304–307 (2008).
[Crossref]

Zhang, C.

Zhang, C. Q.

P. Zhao, H. J. Cong, X. X. Tian, Y. X. Sun, C. Q. Zhang, S. Q. Xia, Z. L. Gao, and X. T. Tao, “Top-Seeded Solution Growth, Structure, Morphology, and Functional Properties of a New Polar Crystal – Cs2TeW3O12,” Cryst. Growth Des. 15(9), 4484–4489 (2015).
[Crossref]

J. J. Zhang, Z. H. Zhang, Y. X. Sun, C. Q. Zhang, and X. T. Tao, “Anisotropic thermal properties of the polar crystal Cs2TeMo3O12,” J. Solid State Chem. 195, 120–124 (2012).
[Crossref]

J. J. Zhang, Z. H. Zhang, Y. X. Sun, C. Q. Zhang, S. J. Zhang, Y. Liu, and X. T. Tao, “MgTeMoO6: A neutral layered material showing strong second-harmonic generation,” J. Mater. Chem. 22(19), 9921–9927 (2012).
[Crossref]

J. J. Zhang, Z. H. Zhang, W. G. Zhang, Q. X. Zheng, Y. X. Sun, C. Q. Zhang, and X. Tao, “Polymorphism of BaTeMo2O9: A New Polar Polymorph and the Phase Transformation,” Chem. Mater. 23(16), 3752–3761 (2011).
[Crossref]

J. J. Zhang, X. T. Tao, Y. X. Sun, Z. H. Zhang, C. Q. Zhang, Z. L. Gao, H. B. Xia, and S. Q. Xia, “Top-Seeded Solution Growth, Morphology, and Properties of a Polar Crystal Cs2TeMo3O12,” Cryst. Growth Des. 11(5), 1863–1868 (2011).
[Crossref]

W. G. Zhang, X. T. Tao, C. Q. Zhang, Z. L. Gao, Y. Z. Zhang, W. T. Yu, X. F. Cheng, X. S. Li, and M. H. Jiang, “Bulk Growth and Characterization of a Novel Nonlinear Optical Crystal BaTeMo2O9,” Cryst. Growth Des. 8(1), 304–307 (2008).
[Crossref]

Zhang, J. J.

X. X. Feng, J. J. Zhang, Z. L. Gao, S. J. Zhang, Y. X. Sun, and X. T. Tao, “Investigation of the second-order nonlinear optical properties of Cs2TeMo3O12 single crystal,” Appl. Phys. Lett. 104(8), 081912 (2014).
[Crossref]

J. J. Zhang, Z. H. Zhang, Y. X. Sun, C. Q. Zhang, S. J. Zhang, Y. Liu, and X. T. Tao, “MgTeMoO6: A neutral layered material showing strong second-harmonic generation,” J. Mater. Chem. 22(19), 9921–9927 (2012).
[Crossref]

J. J. Zhang, Z. H. Zhang, Y. X. Sun, C. Q. Zhang, and X. T. Tao, “Anisotropic thermal properties of the polar crystal Cs2TeMo3O12,” J. Solid State Chem. 195, 120–124 (2012).
[Crossref]

J. J. Zhang, X. T. Tao, Y. X. Sun, Z. H. Zhang, C. Q. Zhang, Z. L. Gao, H. B. Xia, and S. Q. Xia, “Top-Seeded Solution Growth, Morphology, and Properties of a Polar Crystal Cs2TeMo3O12,” Cryst. Growth Des. 11(5), 1863–1868 (2011).
[Crossref]

J. J. Zhang, Z. H. Zhang, W. G. Zhang, Q. X. Zheng, Y. X. Sun, C. Q. Zhang, and X. Tao, “Polymorphism of BaTeMo2O9: A New Polar Polymorph and the Phase Transformation,” Chem. Mater. 23(16), 3752–3761 (2011).
[Crossref]

Zhang, J.-Y.

Zhang, S. J.

X. X. Feng, J. J. Zhang, Z. L. Gao, S. J. Zhang, Y. X. Sun, and X. T. Tao, “Investigation of the second-order nonlinear optical properties of Cs2TeMo3O12 single crystal,” Appl. Phys. Lett. 104(8), 081912 (2014).
[Crossref]

Q. X. Yu, Z. L. Gao, S. J. Zhang, W. G. Zhang, S. P. Wang, and X. T. Tao, “Second order nonlinear properties of monoclinic single crystal BaTeMo2O9,” J. Appl. Phys. 111(1), 013506 (2012).
[Crossref]

J. J. Zhang, Z. H. Zhang, Y. X. Sun, C. Q. Zhang, S. J. Zhang, Y. Liu, and X. T. Tao, “MgTeMoO6: A neutral layered material showing strong second-harmonic generation,” J. Mater. Chem. 22(19), 9921–9927 (2012).
[Crossref]

Zhang, W. G.

Q. X. Yu, Z. L. Gao, S. J. Zhang, W. G. Zhang, S. P. Wang, and X. T. Tao, “Second order nonlinear properties of monoclinic single crystal BaTeMo2O9,” J. Appl. Phys. 111(1), 013506 (2012).
[Crossref]

J. J. Zhang, Z. H. Zhang, W. G. Zhang, Q. X. Zheng, Y. X. Sun, C. Q. Zhang, and X. Tao, “Polymorphism of BaTeMo2O9: A New Polar Polymorph and the Phase Transformation,” Chem. Mater. 23(16), 3752–3761 (2011).
[Crossref]

W. G. Zhang, F. Li, S.-H. Kim, and P. S. Halasyamani, “Top-Seeded Solution Crystal Growth and Functional Properties of a Polar Material–Na2TeW2O9,” Cryst. Growth Des. 10(9), 4091–4095 (2010).
[Crossref]

W. G. Zhang, X. T. Tao, C. Q. Zhang, Z. L. Gao, Y. Z. Zhang, W. T. Yu, X. F. Cheng, X. S. Li, and M. H. Jiang, “Bulk Growth and Characterization of a Novel Nonlinear Optical Crystal BaTeMo2O9,” Cryst. Growth Des. 8(1), 304–307 (2008).
[Crossref]

Zhang, X.

Zhang, Y. Z.

W. G. Zhang, X. T. Tao, C. Q. Zhang, Z. L. Gao, Y. Z. Zhang, W. T. Yu, X. F. Cheng, X. S. Li, and M. H. Jiang, “Bulk Growth and Characterization of a Novel Nonlinear Optical Crystal BaTeMo2O9,” Cryst. Growth Des. 8(1), 304–307 (2008).
[Crossref]

Zhang, Z. H.

J. J. Zhang, Z. H. Zhang, Y. X. Sun, C. Q. Zhang, S. J. Zhang, Y. Liu, and X. T. Tao, “MgTeMoO6: A neutral layered material showing strong second-harmonic generation,” J. Mater. Chem. 22(19), 9921–9927 (2012).
[Crossref]

J. J. Zhang, Z. H. Zhang, Y. X. Sun, C. Q. Zhang, and X. T. Tao, “Anisotropic thermal properties of the polar crystal Cs2TeMo3O12,” J. Solid State Chem. 195, 120–124 (2012).
[Crossref]

J. J. Zhang, Z. H. Zhang, W. G. Zhang, Q. X. Zheng, Y. X. Sun, C. Q. Zhang, and X. Tao, “Polymorphism of BaTeMo2O9: A New Polar Polymorph and the Phase Transformation,” Chem. Mater. 23(16), 3752–3761 (2011).
[Crossref]

J. J. Zhang, X. T. Tao, Y. X. Sun, Z. H. Zhang, C. Q. Zhang, Z. L. Gao, H. B. Xia, and S. Q. Xia, “Top-Seeded Solution Growth, Morphology, and Properties of a Polar Crystal Cs2TeMo3O12,” Cryst. Growth Des. 11(5), 1863–1868 (2011).
[Crossref]

Zhao, B.

Zhao, P.

P. Zhao, H. J. Cong, X. X. Tian, Y. X. Sun, C. Q. Zhang, S. Q. Xia, Z. L. Gao, and X. T. Tao, “Top-Seeded Solution Growth, Structure, Morphology, and Functional Properties of a New Polar Crystal – Cs2TeW3O12,” Cryst. Growth Des. 15(9), 4484–4489 (2015).
[Crossref]

Zheng, Q. X.

J. J. Zhang, Z. H. Zhang, W. G. Zhang, Q. X. Zheng, Y. X. Sun, C. Q. Zhang, and X. Tao, “Polymorphism of BaTeMo2O9: A New Polar Polymorph and the Phase Transformation,” Chem. Mater. 23(16), 3752–3761 (2011).
[Crossref]

Zhu, Y.

Appl. Phys. B (1)

C. T. Chen, G. L. Wang, X. Y. Wang, and Z. Y. Xu, “Deep-UV nonlinear optical crystal KBe2BO3F2– discovery, growth, optical properties and applications,” Appl. Phys. B 97(1), 9–25 (2009).
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Appl. Phys. Lett. (2)

X. X. Feng, J. J. Zhang, Z. L. Gao, S. J. Zhang, Y. X. Sun, and X. T. Tao, “Investigation of the second-order nonlinear optical properties of Cs2TeMo3O12 single crystal,” Appl. Phys. Lett. 104(8), 081912 (2014).
[Crossref]

S. X. Dou, M. H. Jiang, Z. S. Shao, and X. T. Tao, “Maker fringes in biaxial crystals and the nonlinear optical coefficients of thiosemicarbazide cadmium chloride monohydrate,” Appl. Phys. Lett. 54(12), 1101–1103 (1989).
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Chem. Mater. (5)

J. J. Zhang, Z. H. Zhang, W. G. Zhang, Q. X. Zheng, Y. X. Sun, C. Q. Zhang, and X. Tao, “Polymorphism of BaTeMo2O9: A New Polar Polymorph and the Phase Transformation,” Chem. Mater. 23(16), 3752–3761 (2011).
[Crossref]

E. O. Chi, K. M. Ok, Y. Porter, and P. S. Halasyamani, “Na2Te3Mo3O16: A New Molybdenum Tellurite with Second-Harmonic Generating and Pyroelectric Properties,” Chem. Mater. 18(8), 2070–2074 (2006).
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P. S. Halasyamani and K. R. Poeppelmeier, “Noncentrosymmetric oxides,” Chem. Mater. 10(10), 2753–2769 (1998).
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J. Goodey, J. Broussard, and P. S. Halasyamani, “Synthesis, Structure, and Characterization of a New Second-Harmonic-Generating Tellurite: Na2TeW2O9,” Chem. Mater. 14(7), 3174–3180 (2002).
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P. Shiv Halasyamani, “Asymmetric Cation Coordination in Oxide Materials: Influence of Lone-Pair Cations on the Intra-octahedral Distortion in d0 Transition Metals,” Chem. Mater. 16(19), 3586–3592 (2004).
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N. Ye, C. Y. Tu, X. F. Long, and M. C. Hong, “Recent Advances in crystal growth in china: laser, nonlinear optical, and ferroelectric crystals,” Cryst. Growth Des. 10(11), 4672–4681 (2010).
[Crossref]

W. G. Zhang, X. T. Tao, C. Q. Zhang, Z. L. Gao, Y. Z. Zhang, W. T. Yu, X. F. Cheng, X. S. Li, and M. H. Jiang, “Bulk Growth and Characterization of a Novel Nonlinear Optical Crystal BaTeMo2O9,” Cryst. Growth Des. 8(1), 304–307 (2008).
[Crossref]

J. J. Zhang, X. T. Tao, Y. X. Sun, Z. H. Zhang, C. Q. Zhang, Z. L. Gao, H. B. Xia, and S. Q. Xia, “Top-Seeded Solution Growth, Morphology, and Properties of a Polar Crystal Cs2TeMo3O12,” Cryst. Growth Des. 11(5), 1863–1868 (2011).
[Crossref]

P. Zhao, H. J. Cong, X. X. Tian, Y. X. Sun, C. Q. Zhang, S. Q. Xia, Z. L. Gao, and X. T. Tao, “Top-Seeded Solution Growth, Structure, Morphology, and Functional Properties of a New Polar Crystal – Cs2TeW3O12,” Cryst. Growth Des. 15(9), 4484–4489 (2015).
[Crossref]

W. G. Zhang, F. Li, S.-H. Kim, and P. S. Halasyamani, “Top-Seeded Solution Crystal Growth and Functional Properties of a Polar Material–Na2TeW2O9,” Cryst. Growth Des. 10(9), 4091–4095 (2010).
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Ferroelectrics (1)

D. Eimerl, “Electro-optic, linear and nonlinear optical properties of KDP and its isomorphs,” Ferroelectrics 72(1), 95–139 (1987).
[Crossref]

IEEE J. Quantum Electron. (1)

D. A. Roberts, “Simplified characterization of uniaxial and biaxial nonlinear optical crystals: a plea for standardization of nomenclature and conventions,” IEEE J. Quantum Electron. 28(10), 2057–2074 (1992).
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Inorg. Chem. (3)

S. D. Nguyen, S.-H. Kim, and P. S. Halasyamani, “Synthesis, Characterization, and Structure-Property Relationships in Two New Polar Oxides: Zn2(MoO4)(SeO3) and Zn2(MoO4)(TeO3),” Inorg. Chem. 50(11), 5215–5222 (2011).
[Crossref] [PubMed]

J. Yeon, S.-H. Kim, S. D. Nguyen, H. Lee, and P. S. Halasyamani, “Two New Noncentrosymmetric (NCS) Polar Oxides: Syntheses, Characterization, and Structure-Property Relationships in BaMTe2O7 (M = Mg2+ or Zn2+),” Inorg. Chem. 51(4), 2662–2668 (2012).
[Crossref] [PubMed]

S. D. Nguyen and P. S. Halasyamani, “Synthesis, Structure, and Characterization of New Li+-d0-Lone-Pair-Oxides: Noncentrosymmetric Polar Li6(Mo2O5)3(SeO3)6 and Centrosymmetric Li2(MO3)(TeO3) (M = Mo6+ or W6+),” Inorg. Chem. 51(17), 9529–9538 (2012).
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C. F. Sun, C. L. Hu, X. Xu, J. B. Ling, T. Hu, F. Kong, X. F. Long, and J. G. Mao, “BaNbO(IO3)5: A New Polar Material with a Very Large SHG Response,” J. Am. Chem. Soc. 131(27), 9486–9487 (2009).
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S. D. Nguyen, J. Yeon, S.-H. Kim, and P. S. Halasyamani, “BiO(IO3): A New Polar Iodate that Exhibits An Aurivillius-Type (Bi2O2)2+ Layer and a Large SHG Response,” J. Am. Chem. Soc. 133(32), 12422–12425 (2011).
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H. S. Ra, K. M. Ok, and P. S. Halasyamani, “Combining Second-Order Jahn-Teller Distorted Cations to Create Highly Efficient SHG Materials: Synthesis, Characterization, and NLO Properties of BaTeM2O9 (M = Mo6+ or W6+),” J. Am. Chem. Soc. 125(26), 7764–7765 (2003).
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J. Appl. Phys. (1)

Q. X. Yu, Z. L. Gao, S. J. Zhang, W. G. Zhang, S. P. Wang, and X. T. Tao, “Second order nonlinear properties of monoclinic single crystal BaTeMo2O9,” J. Appl. Phys. 111(1), 013506 (2012).
[Crossref]

J. Mater. Chem. (1)

J. J. Zhang, Z. H. Zhang, Y. X. Sun, C. Q. Zhang, S. J. Zhang, Y. Liu, and X. T. Tao, “MgTeMoO6: A neutral layered material showing strong second-harmonic generation,” J. Mater. Chem. 22(19), 9921–9927 (2012).
[Crossref]

J. Opt. Soc. Am. B (1)

J. Solid State Chem. (1)

J. J. Zhang, Z. H. Zhang, Y. X. Sun, C. Q. Zhang, and X. T. Tao, “Anisotropic thermal properties of the polar crystal Cs2TeMo3O12,” J. Solid State Chem. 195, 120–124 (2012).
[Crossref]

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Figures (7)

Fig. 1
Fig. 1 Calculated curves from the Sellmeir fits and dispersion curves of the refractive indices for CTW crystal.
Fig. 2
Fig. 2 The samples for measurements on CTW crystal by the MF technique.
Fig. 3
Fig. 3 Maker Fringes measurement for the NLO coefficients. Theoretical Maker Fringe (a) and experimental Maker Fringe (c) of d32. Theoretical Maker Fringe (b) and Experimental Maker Fringe (d) of d33. Note that the red curves represent the envelope curve.
Fig. 4
Fig. 4 The type-I PM angels versus wavelengths of CTW crystal.
Fig. 5
Fig. 5 Ball-and-stick diagram of CTW in ac-plane. Note that CTW exhibits a two-dimensional layered structure along the c-direction.
Fig. 6
Fig. 6 Thermal diffusivity coefficient versus temperature for CTW and CTM along different crystallographic directions.
Fig. 7
Fig. 7 Ball-and-stick diagram of WO6 octahedron and TeO4 polyhedra in CTW. Note that the red arrows indicate the direction of the distortion of WO6 octahedron and TeO4 polyhedra.

Tables (2)

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Table 1 Refractive Indices for CTW Crystal

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Table 2 Second-order NLO coefficients and the effective NLO coefficients of CTW, CTM, and two common-used crystals at room temperature

Equations (7)

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n o 2 =4.24822+ 0.10569 λ 2 -0.05791 -0 .01715λ 2
n e 2 =3.62986+ 0.0574 λ 2 -0.04271 -0 .00699λ 2
I 2 f(θ)× d ij 2 ×T
d ij(CTW) d 36(KDP) = I 2(CTW) f (θ) (CTW) × f (θ) (KDP) I 2(KDP) × T (KDP) T (CTW)
θ m (I)=arcsin [ ( n 2 e n 1 o ) 2 × ( n 2 o ) 2 ( n 1 o ) 2 ( n 2 o ) 2 ( n 2 e ) 2 ] 0.5
d eff = d 32 ×sin(θ)
Δd= | ( W O 1 )( W O 2A ) | | cos θ 1 | + | ( W O 2 )( W O 1A ) | | cos θ 2 | + | ( W O 3 )( W O 4 ) | | cos θ 3 |

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