Abstract

Metamagnetic transition in FeRh has been subject to many investigations. Several methods have been employed to address various characteristics as they change across this transition, such as SQUID magnetometry, neutron scattering, electrical transport, synchrotron X-rays, scanning tunneling microscopy, magneto-optic Kerr effect, etc. In this paper we investigate the frequency dependent reflectance, which is a fast and easy probe, to find clear and distinct signatures of this transition. To this end, our first principle calculations reveal that the dramatic difference in electronic structure between the ferro- and antiferromagnetic phases of FeRh leads to a characteristic crossover in the energy dependence whereby the reflectivity difference between the two phases changes sign at E=∼0.79 eV (1400 nm). To verify these predictions, we have measured the optical reflectance of FeRh thin films across the metamagnetic transition, and found a close agreement with the predicted effect. These measurements not only confirm the calculated electronic structure of FeRh, but also reveal an effect that can be used for a fast and easy direct detection of the transition by probing the crossover optically in energy space, without resorting to complicated magneto optical probes which only show a signature of the surface magnetism. This also may be used as a unique probe of the dynamics of carriers by temporal studies in different regions, (from energies near the relaxation frequency to those above the plasma frequency).

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    [Crossref]
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    [Crossref]
  22. J. Kudrnovský, V. Drchal, and I. Turek, “Physical properties of FeRh alloys: The antiferromagnetic to ferromagnetic transition,” Phys. Rev. B 91(1), 014435 (2015).
    [Crossref]
  23. R. Y. Gu and V. P. Antropov, “Dominance of the spin-wave contribution to the magnetic phase transition in FeRh,” Phys. Rev. B 72(1), 012403 (2005).
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    [Crossref]
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    [Crossref]
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    [Crossref]
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    [Crossref]
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    [Crossref]
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    [Crossref]
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    [Crossref]

2018 (5)

F. Pressacco, V. Uhlíř, M. Gatti, A. Nicolaou, A. Bendounan, J. A. Arregi, S. K. K. Patel, E. E. Fullerton, D. Krizmancic, and F. Sirotti, “Laser induced phase transition in epitaxial FeRh layers studied by pump-probe valence band photoemission,” Struct. Dyn. 5(3), 034501 (2018).
[Crossref]

S. P. Bennett, A. Herklotz, C. D. Cress, A. Ievlev, C. M. Rouleau, I. I. Mazin, and V. Lauter, “Magnetic order multilayering in FeRh thin films by He-Ion irradiation,” Mater. Res. Lett. 6(1), 106–112 (2018).
[Crossref]

R. C. Temple, T. P. Almeida, J. R. Massey, K. Fallon, R. Lamb, S. A. Morley, F. Maccherozzi, S. S. Dhesi, D. McGrouther, S. McVitie, T. A. Moore, and C. H. Marrows, “Antiferromagnetic-ferromagnetic phase domain development in nanopatterned FeRh islands,” Phys. Rev. Mater. 2(10), 104406 (2018).
[Crossref]

S. P. Bennett, A. Herklotz, C. D. Cress, A. Ievlev, C. M. Rouleau, I. I. Mazin, and V. Lauter, “Magnetic order multilayering in FeRh thin films by the He-ion irradiation,” Mater. Res. Lett. 6(1), 106–112 (2018).
[Crossref]

T. P. Almeida, R. Temple, J. Massey, K. Fallon, G. Paterson, T. Moore, D. McGrouther, C. H. Marrows, and S. McVitie, “Quantitative Differential Phase Contrast Imaging of the Magnetostructural Transition and Current-driven Motion of Domain Walls in FeRh Thin Films,” Microsc. Microanal. 24(S1), 936–937 (2018).
[Crossref]

2017 (4)

C. W. Barton, T. A. Ostler, D. Huskisson, C. J. Kinane, S. J. Haigh, G. Hrkac, and T. Thomson, “Substrate Induced Strain Field in FeRh Epilayers Grown on Single Crystal MgO (001) Substrates,” Sci. Rep. 7(1), 44397 (2017).
[Crossref]

T. A. Ostler, C. Barton, T. Thomson, and G. Hrkac, “Modeling the thickness dependence of the magnetic phase transition temperature in thin FeRh films,” Phys. Rev. B 95(6), 064415 (2017).
[Crossref]

S. Mankovsky, S. Polesya, K. Chadova, H. Ebert, J. B. Staunton, T. Gruenbaum, M. A. W. Schoen, C. H. Back, X. Z. Chen, and C. Song, “Temperature-dependent transport properties of FeRh,” Phys. Rev. B 95(15), 155139 (2017).
[Crossref]

A. A. Ünal, A. Parabas, A. Arora, J. Ehrler, C. Barton, S. Valencia, R. Bali, T. Thomson, F. Yildiz, and F. Kronast, “Laser-driven formation of transient local ferromagnetism in FeRh thin films,” Ultramicroscopy 183, 104–108 (2017).
[Crossref]

2016 (3)

V. Saidl, M. Brajer, L. Horák, H. Reichlová, K. Výborný, M. Veis, T. Janda, F. Trojánek, M. Maryško, I. Fina, X. Marti, T. Jungwirth, and P. Němec, “Investigation of magneto-structural phase transition in FeRh by reflectivity and transmittance measurements in visible and near-infrared spectral region,” New J. Phys. 18(8), 083017 (2016).
[Crossref]

S. P. Bennett, A. T. Wong, A. Glavic, A. Herklotz, C. Urban, I. Valmianski, M. D. Biegalski, H. M. Christen, T. Z. Ward, and V. Lauter, “Giant Controllable Magnetization Changes Induced by Structural Phase Transitions in a Metamagnetic Artificial Multiferroic,” Sci. Rep. 6(1), 22708 (2016).
[Crossref]

V. Uhlíř, J. A. Arregi, and E. E. Fullerton, “Colossal magnetic phase transition asymmetry in mesoscale FeRh stripes,” Nat. Commun. 7(1), 13113 (2016).
[Crossref]

2015 (4)

Y. Lee, Z. Q. Liu, J. T. Heron, J. D. Clarkson, J. Hong, C. Ko, M. D. Biegalski, U. Aschauer, S. L. Hsu, M. E. Nowakowski, J. Wu, H. M. Christen, S. Salahuddin, J. B. Bokor, N. A. Spaldin, D. G. Schlom, and R. Ramesh, “Large resistivity modulation in mixed-phase metallic systems,” Nat. Commun. 6(1), 5959 (2015).
[Crossref]

S. P. Bennett, H. Ambaye, H. Lee, P. LeClair, G. J. Mankey, and V. Lauter, “Direct Evidence of Anomalous Interfacial Magnetization in Metamagnetic Pd doped FeRh Thin Films,” Sci. Rep. 5(1), 9142 (2015).
[Crossref]

J. Kudrnovský, V. Drchal, and I. Turek, “Physical properties of FeRh alloys: The antiferromagnetic to ferromagnetic transition,” Phys. Rev. B 91(1), 014435 (2015).
[Crossref]

L. H. Lewis, R. Barua, and B. Lejeune, “Developing magnetofunctionality: Coupled structural and magnetic phase transition in AlFe2B2,” J. Alloys Compd. 650, 482–488 (2015).
[Crossref]

2014 (4)

J. B. Staunton, R. Banerjee, M. dos, S. Dias, A. Deak, and L. Szunyogh, “Fluctuating local moments, itinerant electrons, and the magnetocaloric effect: Compositional hypersensitivity of FeRh,” Phys. Rev. B 89(5), 054427 (2014).
[Crossref]

I. Suzuki, M. Itoh, and T. Taniyama, “Elastically controlled magnetic phase transition in Ga-FeRh/BaTiO3(001) heterostructure,” Appl. Phys. Lett. 104(2), 022401 (2014).
[Crossref]

R. O. Cherifi, V. Ivanovskaya, L. C. Phillips, A. Zobelli, I. C. Infante, E. Jacquet, V. Garcia, S. Fusil, P. R. Briddon, N. Guiblin, A. Mougin, A. A. Ünal, F. Kronast, S. Valencia, B. Dkhil, A. Barthélémy, and M. Bibes, “Electric-field control of magnetic order above room temperature,” Nat. Mater. 13(4), 345–351 (2014).
[Crossref]

X. Marti, I. Fina, C. Frontera, J. Liu, P. Wadley, Q. He, R. J. Paull, J. D. Clarkson, J. Kudrnovský, I. Turek, J. Kuneš, D. Yi, J. Chu, C. T. Nelson, L. You, E. Arenholz, S. Salahuddin, J. Fontcuberta, T. Jungwirth, and R. Ramesh, “Room-temperature antiferromagnetic memory resistor,” Nat. Mater. 13(4), 367–374 (2014).
[Crossref]

2013 (1)

M. Loving, F. Jimenez-Villacorta, B. Kaeswurm, D. A. Arena, C. H. Marrows, and L. H. Lewis, “Structural evidence for stabilized ferromagnetism in epitaxial FeRh nanoislands,” J. Phys. D: Appl. Phys. 46(16), 162002 (2013).
[Crossref]

2012 (1)

S. O. Mariager, F. Pressacco, G. Ingold, A. Caviezel, E. Möhr-Vorobeva, P. Beaud, S. L. Johnson, C. J. Milne, E. Mancini, S. Moyerman, E. E. Fullerton, R. Feidenhans’l, C. H. Back, and C. Quitmann, “Structural and Magnetic Dynamics of a Laser Induced Phase Transition in FeRh,” Phys. Rev. Lett. 108(8), 087201 (2012).
[Crossref]

2011 (3)

L. M. Sandratskii and P. Mavropoulos, “Magnetic excitations and femtomagnetism of FeRh: A first-principles study,” Phys. Rev. B 83(17), 174408 (2011).
[Crossref]

L. M. Sandratskii and P. Mavropoulos, “Magnetic excitations and femtomagnetism of FeRh: A first-principles study,” Phys. Rev. B: Condens. Matter Mater. Phys. 83(17), 174408 (2011).
[Crossref]

M. Sharma, H. M. Aarbogh, J. U. Thiele, S. Maat, E. E. Fullerton, and C. Leighton, “Magnetotransport properties of epitaxial MgO(001)/FeRh films across the antiferromagnet to ferromagnet transition,” J. Appl. Phys. 109(8), 083913 (2011).
[Crossref]

2010 (2)

R. Fan, C. J. Kinane, T. R. Charlton, R. Dorner, M. Ali, M. A. De Vries, R. M. D. Brydson, C. H. Marrows, B. J. Hickey, D. A. Arena, B. K. Tanner, G. Nisbet, and S. Langridge, “Ferromagnetism at the interfaces of antiferromagnetic FeRh epilayers,” Phys. Rev. B: Condens. Matter Mater. Phys. 82(18), 184418 (2010).
[Crossref]

I. Radu, C. Stamm, N. Pontius, T. Kachel, P. Ramm, J.-U. Thiele, H. A. Dürr, and C. H. Back, “Laser-induced generation and quenching of magnetization on FeRh studied with time-resolved x-ray magnetic circular dichroism,” Phys. Rev. B 81(10), 104415 (2010).
[Crossref]

2005 (1)

R. Y. Gu and V. P. Antropov, “Dominance of the spin-wave contribution to the magnetic phase transition in FeRh,” Phys. Rev. B 72(1), 012403 (2005).
[Crossref]

2004 (1)

G. Ju, J. Hohlfeld, B. Bergman, R. J. M. van de Veerdonk, O. N. Mryasov, J.-Y. Kim, X. Wu, D. Weller, and B. Koopmans, “Ultrafast Generation of Ferromagnetic Order via a Laser-Induced Phase Transformation in FeRh Thin Films,” Phys. Rev. Lett. 93(19), 197403 (2004).
[Crossref]

1996 (1)

J. P. Perdew, K. Burke, and M. Ernzerhof, “Generalized Gradient Approximation Made Simple,” Phys. Rev. Lett. 77(18), 3865–3868 (1996).
[Crossref]

1995 (1)

J. Y. Rhee and D. W. Lynch, “Optical properties of Fe-Rh alloys,” Phys. Rev. B 51(3), 1926–1927 (1995).
[Crossref]

1993 (1)

H. Miyajima, S. Yuasa, and Y. Otani, “First-Order Magnetic Phase Transitions Observed in bct FeRh–Pt, Pd Systems,” Jpn. J. Appl. Phys. 32(S3), 232 (1993).
[Crossref]

1988 (1)

L.-Y. Chen and D. W. Lynch, “Ellipsometric studies of magnetic phase transitions of Fe-Rh alloys,” Phys. Rev. B 37(18), 10503–10509 (1988).
[Crossref]

1983 (1)

M. A. Khan, C. Koenig, and R. Riedinger, “Interband dielectric constants in antiferromagnetic, ferromagnetic and paramagnetic phases of FeRh,” J. Phys. F: Met. Phys. 13(8), L159–L164 (1983).
[Crossref]

1982 (1)

C. Koenig, “Self-consistent band structure of paramagnetic, ferromagnetic and antiferromagnetic ordered FeRh,” J. Phys. F: Met. Phys. 12(6), 1123–1137 (1982).
[Crossref]

1967 (1)

J. M. Lommel and J. S. Kouvel, “Effects of mechanical and thermal treatment on the structure and magnetic transitions in FeRh,” J. Appl. Phys. 38(3), 1263–1264 (1967).
[Crossref]

1966 (1)

J. M. Lommel, “Magnetic and electrical properties of FeRh thin films,” J. Appl. Phys. 37(3), 1483–1484 (1966).
[Crossref]

1962 (1)

J. S. Kouvel and C. C. Hartelius, “Anomalous magnetic moments and transformations in the ordered alloy FeRh,” J. Appl. Phys. 33(3), 1343–1344 (1962).
[Crossref]

Aarbogh, H. M.

M. Sharma, H. M. Aarbogh, J. U. Thiele, S. Maat, E. E. Fullerton, and C. Leighton, “Magnetotransport properties of epitaxial MgO(001)/FeRh films across the antiferromagnet to ferromagnet transition,” J. Appl. Phys. 109(8), 083913 (2011).
[Crossref]

Ali, M.

R. Fan, C. J. Kinane, T. R. Charlton, R. Dorner, M. Ali, M. A. De Vries, R. M. D. Brydson, C. H. Marrows, B. J. Hickey, D. A. Arena, B. K. Tanner, G. Nisbet, and S. Langridge, “Ferromagnetism at the interfaces of antiferromagnetic FeRh epilayers,” Phys. Rev. B: Condens. Matter Mater. Phys. 82(18), 184418 (2010).
[Crossref]

Almeida, T. P.

R. C. Temple, T. P. Almeida, J. R. Massey, K. Fallon, R. Lamb, S. A. Morley, F. Maccherozzi, S. S. Dhesi, D. McGrouther, S. McVitie, T. A. Moore, and C. H. Marrows, “Antiferromagnetic-ferromagnetic phase domain development in nanopatterned FeRh islands,” Phys. Rev. Mater. 2(10), 104406 (2018).
[Crossref]

T. P. Almeida, R. Temple, J. Massey, K. Fallon, G. Paterson, T. Moore, D. McGrouther, C. H. Marrows, and S. McVitie, “Quantitative Differential Phase Contrast Imaging of the Magnetostructural Transition and Current-driven Motion of Domain Walls in FeRh Thin Films,” Microsc. Microanal. 24(S1), 936–937 (2018).
[Crossref]

Ambaye, H.

S. P. Bennett, H. Ambaye, H. Lee, P. LeClair, G. J. Mankey, and V. Lauter, “Direct Evidence of Anomalous Interfacial Magnetization in Metamagnetic Pd doped FeRh Thin Films,” Sci. Rep. 5(1), 9142 (2015).
[Crossref]

Antropov, V. P.

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C. W. Barton, T. A. Ostler, D. Huskisson, C. J. Kinane, S. J. Haigh, G. Hrkac, and T. Thomson, “Substrate Induced Strain Field in FeRh Epilayers Grown on Single Crystal MgO (001) Substrates,” Sci. Rep. 7(1), 44397 (2017).
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S. P. Bennett, A. Herklotz, C. D. Cress, A. Ievlev, C. M. Rouleau, I. I. Mazin, and V. Lauter, “Magnetic order multilayering in FeRh thin films by He-Ion irradiation,” Mater. Res. Lett. 6(1), 106–112 (2018).
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C. W. Barton, T. A. Ostler, D. Huskisson, C. J. Kinane, S. J. Haigh, G. Hrkac, and T. Thomson, “Substrate Induced Strain Field in FeRh Epilayers Grown on Single Crystal MgO (001) Substrates,” Sci. Rep. 7(1), 44397 (2017).
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R. Fan, C. J. Kinane, T. R. Charlton, R. Dorner, M. Ali, M. A. De Vries, R. M. D. Brydson, C. H. Marrows, B. J. Hickey, D. A. Arena, B. K. Tanner, G. Nisbet, and S. Langridge, “Ferromagnetism at the interfaces of antiferromagnetic FeRh epilayers,” Phys. Rev. B: Condens. Matter Mater. Phys. 82(18), 184418 (2010).
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C. Koenig, “Self-consistent band structure of paramagnetic, ferromagnetic and antiferromagnetic ordered FeRh,” J. Phys. F: Met. Phys. 12(6), 1123–1137 (1982).
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F. Pressacco, V. Uhlíř, M. Gatti, A. Nicolaou, A. Bendounan, J. A. Arregi, S. K. K. Patel, E. E. Fullerton, D. Krizmancic, and F. Sirotti, “Laser induced phase transition in epitaxial FeRh layers studied by pump-probe valence band photoemission,” Struct. Dyn. 5(3), 034501 (2018).
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S. P. Bennett, A. Herklotz, C. D. Cress, A. Ievlev, C. M. Rouleau, I. I. Mazin, and V. Lauter, “Magnetic order multilayering in FeRh thin films by the He-ion irradiation,” Mater. Res. Lett. 6(1), 106–112 (2018).
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S. P. Bennett, A. Herklotz, C. D. Cress, A. Ievlev, C. M. Rouleau, I. I. Mazin, and V. Lauter, “Magnetic order multilayering in FeRh thin films by He-Ion irradiation,” Mater. Res. Lett. 6(1), 106–112 (2018).
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S. P. Bennett, A. T. Wong, A. Glavic, A. Herklotz, C. Urban, I. Valmianski, M. D. Biegalski, H. M. Christen, T. Z. Ward, and V. Lauter, “Giant Controllable Magnetization Changes Induced by Structural Phase Transitions in a Metamagnetic Artificial Multiferroic,” Sci. Rep. 6(1), 22708 (2016).
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S. P. Bennett, H. Ambaye, H. Lee, P. LeClair, G. J. Mankey, and V. Lauter, “Direct Evidence of Anomalous Interfacial Magnetization in Metamagnetic Pd doped FeRh Thin Films,” Sci. Rep. 5(1), 9142 (2015).
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S. O. Mariager, L. Le Guyader, M. Buzzi, G. Ingold, and C. Quitmann, “Imaging the antiferromagnetic to ferromagnetic first order phase transition of FeRh,” (2013).

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S. P. Bennett, H. Ambaye, H. Lee, P. LeClair, G. J. Mankey, and V. Lauter, “Direct Evidence of Anomalous Interfacial Magnetization in Metamagnetic Pd doped FeRh Thin Films,” Sci. Rep. 5(1), 9142 (2015).
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Lee, H.

S. P. Bennett, H. Ambaye, H. Lee, P. LeClair, G. J. Mankey, and V. Lauter, “Direct Evidence of Anomalous Interfacial Magnetization in Metamagnetic Pd doped FeRh Thin Films,” Sci. Rep. 5(1), 9142 (2015).
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M. Sharma, H. M. Aarbogh, J. U. Thiele, S. Maat, E. E. Fullerton, and C. Leighton, “Magnetotransport properties of epitaxial MgO(001)/FeRh films across the antiferromagnet to ferromagnet transition,” J. Appl. Phys. 109(8), 083913 (2011).
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X. Marti, I. Fina, C. Frontera, J. Liu, P. Wadley, Q. He, R. J. Paull, J. D. Clarkson, J. Kudrnovský, I. Turek, J. Kuneš, D. Yi, J. Chu, C. T. Nelson, L. You, E. Arenholz, S. Salahuddin, J. Fontcuberta, T. Jungwirth, and R. Ramesh, “Room-temperature antiferromagnetic memory resistor,” Nat. Mater. 13(4), 367–374 (2014).
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L. M. Sandratskii and P. Mavropoulos, “Magnetic excitations and femtomagnetism of FeRh: A first-principles study,” Phys. Rev. B: Condens. Matter Mater. Phys. 83(17), 174408 (2011).
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L. M. Sandratskii and P. Mavropoulos, “Magnetic excitations and femtomagnetism of FeRh: A first-principles study,” Phys. Rev. B 83(17), 174408 (2011).
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Y. Lee, Z. Q. Liu, J. T. Heron, J. D. Clarkson, J. Hong, C. Ko, M. D. Biegalski, U. Aschauer, S. L. Hsu, M. E. Nowakowski, J. Wu, H. M. Christen, S. Salahuddin, J. B. Bokor, N. A. Spaldin, D. G. Schlom, and R. Ramesh, “Large resistivity modulation in mixed-phase metallic systems,” Nat. Commun. 6(1), 5959 (2015).
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Sharma, M.

M. Sharma, H. M. Aarbogh, J. U. Thiele, S. Maat, E. E. Fullerton, and C. Leighton, “Magnetotransport properties of epitaxial MgO(001)/FeRh films across the antiferromagnet to ferromagnet transition,” J. Appl. Phys. 109(8), 083913 (2011).
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Sirotti, F.

F. Pressacco, V. Uhlíř, M. Gatti, A. Nicolaou, A. Bendounan, J. A. Arregi, S. K. K. Patel, E. E. Fullerton, D. Krizmancic, and F. Sirotti, “Laser induced phase transition in epitaxial FeRh layers studied by pump-probe valence band photoemission,” Struct. Dyn. 5(3), 034501 (2018).
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S. Mankovsky, S. Polesya, K. Chadova, H. Ebert, J. B. Staunton, T. Gruenbaum, M. A. W. Schoen, C. H. Back, X. Z. Chen, and C. Song, “Temperature-dependent transport properties of FeRh,” Phys. Rev. B 95(15), 155139 (2017).
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Y. Lee, Z. Q. Liu, J. T. Heron, J. D. Clarkson, J. Hong, C. Ko, M. D. Biegalski, U. Aschauer, S. L. Hsu, M. E. Nowakowski, J. Wu, H. M. Christen, S. Salahuddin, J. B. Bokor, N. A. Spaldin, D. G. Schlom, and R. Ramesh, “Large resistivity modulation in mixed-phase metallic systems,” Nat. Commun. 6(1), 5959 (2015).
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S. Mankovsky, S. Polesya, K. Chadova, H. Ebert, J. B. Staunton, T. Gruenbaum, M. A. W. Schoen, C. H. Back, X. Z. Chen, and C. Song, “Temperature-dependent transport properties of FeRh,” Phys. Rev. B 95(15), 155139 (2017).
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J. B. Staunton, R. Banerjee, M. dos, S. Dias, A. Deak, and L. Szunyogh, “Fluctuating local moments, itinerant electrons, and the magnetocaloric effect: Compositional hypersensitivity of FeRh,” Phys. Rev. B 89(5), 054427 (2014).
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I. Suzuki, M. Itoh, and T. Taniyama, “Elastically controlled magnetic phase transition in Ga-FeRh/BaTiO3(001) heterostructure,” Appl. Phys. Lett. 104(2), 022401 (2014).
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J. B. Staunton, R. Banerjee, M. dos, S. Dias, A. Deak, and L. Szunyogh, “Fluctuating local moments, itinerant electrons, and the magnetocaloric effect: Compositional hypersensitivity of FeRh,” Phys. Rev. B 89(5), 054427 (2014).
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I. Suzuki, M. Itoh, and T. Taniyama, “Elastically controlled magnetic phase transition in Ga-FeRh/BaTiO3(001) heterostructure,” Appl. Phys. Lett. 104(2), 022401 (2014).
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M. Sharma, H. M. Aarbogh, J. U. Thiele, S. Maat, E. E. Fullerton, and C. Leighton, “Magnetotransport properties of epitaxial MgO(001)/FeRh films across the antiferromagnet to ferromagnet transition,” J. Appl. Phys. 109(8), 083913 (2011).
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Thiele, J.-U.

I. Radu, C. Stamm, N. Pontius, T. Kachel, P. Ramm, J.-U. Thiele, H. A. Dürr, and C. H. Back, “Laser-induced generation and quenching of magnetization on FeRh studied with time-resolved x-ray magnetic circular dichroism,” Phys. Rev. B 81(10), 104415 (2010).
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A. A. Ünal, A. Parabas, A. Arora, J. Ehrler, C. Barton, S. Valencia, R. Bali, T. Thomson, F. Yildiz, and F. Kronast, “Laser-driven formation of transient local ferromagnetism in FeRh thin films,” Ultramicroscopy 183, 104–108 (2017).
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J. Kudrnovský, V. Drchal, and I. Turek, “Physical properties of FeRh alloys: The antiferromagnetic to ferromagnetic transition,” Phys. Rev. B 91(1), 014435 (2015).
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X. Marti, I. Fina, C. Frontera, J. Liu, P. Wadley, Q. He, R. J. Paull, J. D. Clarkson, J. Kudrnovský, I. Turek, J. Kuneš, D. Yi, J. Chu, C. T. Nelson, L. You, E. Arenholz, S. Salahuddin, J. Fontcuberta, T. Jungwirth, and R. Ramesh, “Room-temperature antiferromagnetic memory resistor,” Nat. Mater. 13(4), 367–374 (2014).
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Uhlír, V.

F. Pressacco, V. Uhlíř, M. Gatti, A. Nicolaou, A. Bendounan, J. A. Arregi, S. K. K. Patel, E. E. Fullerton, D. Krizmancic, and F. Sirotti, “Laser induced phase transition in epitaxial FeRh layers studied by pump-probe valence band photoemission,” Struct. Dyn. 5(3), 034501 (2018).
[Crossref]

V. Uhlíř, J. A. Arregi, and E. E. Fullerton, “Colossal magnetic phase transition asymmetry in mesoscale FeRh stripes,” Nat. Commun. 7(1), 13113 (2016).
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A. A. Ünal, A. Parabas, A. Arora, J. Ehrler, C. Barton, S. Valencia, R. Bali, T. Thomson, F. Yildiz, and F. Kronast, “Laser-driven formation of transient local ferromagnetism in FeRh thin films,” Ultramicroscopy 183, 104–108 (2017).
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R. O. Cherifi, V. Ivanovskaya, L. C. Phillips, A. Zobelli, I. C. Infante, E. Jacquet, V. Garcia, S. Fusil, P. R. Briddon, N. Guiblin, A. Mougin, A. A. Ünal, F. Kronast, S. Valencia, B. Dkhil, A. Barthélémy, and M. Bibes, “Electric-field control of magnetic order above room temperature,” Nat. Mater. 13(4), 345–351 (2014).
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R. O. Cherifi, V. Ivanovskaya, L. C. Phillips, A. Zobelli, I. C. Infante, E. Jacquet, V. Garcia, S. Fusil, P. R. Briddon, N. Guiblin, A. Mougin, A. A. Ünal, F. Kronast, S. Valencia, B. Dkhil, A. Barthélémy, and M. Bibes, “Electric-field control of magnetic order above room temperature,” Nat. Mater. 13(4), 345–351 (2014).
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S. P. Bennett, A. T. Wong, A. Glavic, A. Herklotz, C. Urban, I. Valmianski, M. D. Biegalski, H. M. Christen, T. Z. Ward, and V. Lauter, “Giant Controllable Magnetization Changes Induced by Structural Phase Transitions in a Metamagnetic Artificial Multiferroic,” Sci. Rep. 6(1), 22708 (2016).
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G. Ju, J. Hohlfeld, B. Bergman, R. J. M. van de Veerdonk, O. N. Mryasov, J.-Y. Kim, X. Wu, D. Weller, and B. Koopmans, “Ultrafast Generation of Ferromagnetic Order via a Laser-Induced Phase Transformation in FeRh Thin Films,” Phys. Rev. Lett. 93(19), 197403 (2004).
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V. Saidl, M. Brajer, L. Horák, H. Reichlová, K. Výborný, M. Veis, T. Janda, F. Trojánek, M. Maryško, I. Fina, X. Marti, T. Jungwirth, and P. Němec, “Investigation of magneto-structural phase transition in FeRh by reflectivity and transmittance measurements in visible and near-infrared spectral region,” New J. Phys. 18(8), 083017 (2016).
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V. Saidl, M. Brajer, L. Horák, H. Reichlová, K. Výborný, M. Veis, T. Janda, F. Trojánek, M. Maryško, I. Fina, X. Marti, T. Jungwirth, and P. Němec, “Investigation of magneto-structural phase transition in FeRh by reflectivity and transmittance measurements in visible and near-infrared spectral region,” New J. Phys. 18(8), 083017 (2016).
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X. Marti, I. Fina, C. Frontera, J. Liu, P. Wadley, Q. He, R. J. Paull, J. D. Clarkson, J. Kudrnovský, I. Turek, J. Kuneš, D. Yi, J. Chu, C. T. Nelson, L. You, E. Arenholz, S. Salahuddin, J. Fontcuberta, T. Jungwirth, and R. Ramesh, “Room-temperature antiferromagnetic memory resistor,” Nat. Mater. 13(4), 367–374 (2014).
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Ward, T. Z.

S. P. Bennett, A. T. Wong, A. Glavic, A. Herklotz, C. Urban, I. Valmianski, M. D. Biegalski, H. M. Christen, T. Z. Ward, and V. Lauter, “Giant Controllable Magnetization Changes Induced by Structural Phase Transitions in a Metamagnetic Artificial Multiferroic,” Sci. Rep. 6(1), 22708 (2016).
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Weller, D.

G. Ju, J. Hohlfeld, B. Bergman, R. J. M. van de Veerdonk, O. N. Mryasov, J.-Y. Kim, X. Wu, D. Weller, and B. Koopmans, “Ultrafast Generation of Ferromagnetic Order via a Laser-Induced Phase Transformation in FeRh Thin Films,” Phys. Rev. Lett. 93(19), 197403 (2004).
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S. P. Bennett, A. T. Wong, A. Glavic, A. Herklotz, C. Urban, I. Valmianski, M. D. Biegalski, H. M. Christen, T. Z. Ward, and V. Lauter, “Giant Controllable Magnetization Changes Induced by Structural Phase Transitions in a Metamagnetic Artificial Multiferroic,” Sci. Rep. 6(1), 22708 (2016).
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Y. Lee, Z. Q. Liu, J. T. Heron, J. D. Clarkson, J. Hong, C. Ko, M. D. Biegalski, U. Aschauer, S. L. Hsu, M. E. Nowakowski, J. Wu, H. M. Christen, S. Salahuddin, J. B. Bokor, N. A. Spaldin, D. G. Schlom, and R. Ramesh, “Large resistivity modulation in mixed-phase metallic systems,” Nat. Commun. 6(1), 5959 (2015).
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Wu, X.

G. Ju, J. Hohlfeld, B. Bergman, R. J. M. van de Veerdonk, O. N. Mryasov, J.-Y. Kim, X. Wu, D. Weller, and B. Koopmans, “Ultrafast Generation of Ferromagnetic Order via a Laser-Induced Phase Transformation in FeRh Thin Films,” Phys. Rev. Lett. 93(19), 197403 (2004).
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X. Marti, I. Fina, C. Frontera, J. Liu, P. Wadley, Q. He, R. J. Paull, J. D. Clarkson, J. Kudrnovský, I. Turek, J. Kuneš, D. Yi, J. Chu, C. T. Nelson, L. You, E. Arenholz, S. Salahuddin, J. Fontcuberta, T. Jungwirth, and R. Ramesh, “Room-temperature antiferromagnetic memory resistor,” Nat. Mater. 13(4), 367–374 (2014).
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Yildiz, F.

A. A. Ünal, A. Parabas, A. Arora, J. Ehrler, C. Barton, S. Valencia, R. Bali, T. Thomson, F. Yildiz, and F. Kronast, “Laser-driven formation of transient local ferromagnetism in FeRh thin films,” Ultramicroscopy 183, 104–108 (2017).
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X. Marti, I. Fina, C. Frontera, J. Liu, P. Wadley, Q. He, R. J. Paull, J. D. Clarkson, J. Kudrnovský, I. Turek, J. Kuneš, D. Yi, J. Chu, C. T. Nelson, L. You, E. Arenholz, S. Salahuddin, J. Fontcuberta, T. Jungwirth, and R. Ramesh, “Room-temperature antiferromagnetic memory resistor,” Nat. Mater. 13(4), 367–374 (2014).
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H. Miyajima, S. Yuasa, and Y. Otani, “First-Order Magnetic Phase Transitions Observed in bct FeRh–Pt, Pd Systems,” Jpn. J. Appl. Phys. 32(S3), 232 (1993).
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I. Suzuki, M. Itoh, and T. Taniyama, “Elastically controlled magnetic phase transition in Ga-FeRh/BaTiO3(001) heterostructure,” Appl. Phys. Lett. 104(2), 022401 (2014).
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T. P. Almeida, R. Temple, J. Massey, K. Fallon, G. Paterson, T. Moore, D. McGrouther, C. H. Marrows, and S. McVitie, “Quantitative Differential Phase Contrast Imaging of the Magnetostructural Transition and Current-driven Motion of Domain Walls in FeRh Thin Films,” Microsc. Microanal. 24(S1), 936–937 (2018).
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Y. Lee, Z. Q. Liu, J. T. Heron, J. D. Clarkson, J. Hong, C. Ko, M. D. Biegalski, U. Aschauer, S. L. Hsu, M. E. Nowakowski, J. Wu, H. M. Christen, S. Salahuddin, J. B. Bokor, N. A. Spaldin, D. G. Schlom, and R. Ramesh, “Large resistivity modulation in mixed-phase metallic systems,” Nat. Commun. 6(1), 5959 (2015).
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R. O. Cherifi, V. Ivanovskaya, L. C. Phillips, A. Zobelli, I. C. Infante, E. Jacquet, V. Garcia, S. Fusil, P. R. Briddon, N. Guiblin, A. Mougin, A. A. Ünal, F. Kronast, S. Valencia, B. Dkhil, A. Barthélémy, and M. Bibes, “Electric-field control of magnetic order above room temperature,” Nat. Mater. 13(4), 345–351 (2014).
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V. Saidl, M. Brajer, L. Horák, H. Reichlová, K. Výborný, M. Veis, T. Janda, F. Trojánek, M. Maryško, I. Fina, X. Marti, T. Jungwirth, and P. Němec, “Investigation of magneto-structural phase transition in FeRh by reflectivity and transmittance measurements in visible and near-infrared spectral region,” New J. Phys. 18(8), 083017 (2016).
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L. M. Sandratskii and P. Mavropoulos, “Magnetic excitations and femtomagnetism of FeRh: A first-principles study,” Phys. Rev. B 83(17), 174408 (2011).
[Crossref]

I. Radu, C. Stamm, N. Pontius, T. Kachel, P. Ramm, J.-U. Thiele, H. A. Dürr, and C. H. Back, “Laser-induced generation and quenching of magnetization on FeRh studied with time-resolved x-ray magnetic circular dichroism,” Phys. Rev. B 81(10), 104415 (2010).
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S. P. Bennett, A. T. Wong, A. Glavic, A. Herklotz, C. Urban, I. Valmianski, M. D. Biegalski, H. M. Christen, T. Z. Ward, and V. Lauter, “Giant Controllable Magnetization Changes Induced by Structural Phase Transitions in a Metamagnetic Artificial Multiferroic,” Sci. Rep. 6(1), 22708 (2016).
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Figures (5)

Fig. 1.
Fig. 1. Calculated density of states (DOS) for (a) the antiferromagnetic phase and (b) the ferromagnetic phase of FeRh. One can see in the AF plot a pseudogap between ∼-0.45 and -0.08 eV, the states below being of the t2 g, and above of the eg character. In the FM plot, t2 g and eg states are not well separated in the majority channel; the eg states start roughly above -0.4 eV and extend to ∼2 eV, while the t2 g ones span an interval between ∼-5.5 and -1 eV.
Fig. 2.
Fig. 2. (a) Calculated optical conductivity assuming the relaxation rate 1/γ is 0.2 eV for both cases. (b) Corresponding reflectivity, with the parameters as listed in the legend.
Fig. 3.
Fig. 3. Magneto-Optic Kerr Effect (MOKE) measurements of an FeRh film (a) Kerr rotation as a function of applied magnetic field H at temperatures from below the transition (87°C)) heating to above the transition (127°C)) The data at 87°C is the raw data without background subtraction (b) Saturation Kerr rotation (taken at H = 1250 Oe) as a function of temperature heating and cooling through the transition to display the temperature hysteresis.
Fig. 4.
Fig. 4. Experimentally obtained CW laser reflectivity measurements of the metamagnetic transition measured at three different laser energies (a) 0.62 eV, (b) 0.80 eV and (c) 1.96eV
Fig. 5.
Fig. 5. Spectral reflectance measurements taken as a function of temperature across the metamagnetic transition with zero applied H-field. (a)&(b) Comparison between theoretically simulated (also shown in Fig. 4(d)) and experimentally acquired spectral reflectance of both phases. (c) Experimentally acquired reflectance as a function of temperature starting at high temperature, 150°C, and cooling to low temperature, 20°C. (d) Experimentally acquired spectral reflectance as a function of temperature starting at low temperature, 20°C, and heating to high temperature, 150°C. The lack of a change in the spectrum until the temperature reaches 120°C for the cooling case in (c), as opposed to spectral changes starting as high as 135°C for the heating case in (d), clarify the expected thermal hysteresis of the metamagnetic transition shown by MOKE in Fig. 3. (e) Plot showing ΔR normalized to R taken at temperatures ranging from 20°C - 150°C for photon energies ranging from 0.52 eV – 1.24 eV delineated by colors, marker shapes and corresponding labels. Shaded markers are points taken on heating while open markers indicate points taken on cooling.

Equations (2)

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R 1 2 2 ω / σ
R 1 2 γ ω p = 1 2 ω p / σ

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